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ISSN 1990-7508, Biochemistry (Moscow), Supplement Series B: Biomedical Chemistry, 2019, Vol. 13, No. 3, pp. 228–236. © Pleiades Publishing, Ltd., 2019.
Russian Text © The Author(s), 2019, published in Biomeditsinskaya Khimiya.
Computer-Aided Xenobiotic Toxicity Prediction Taking into Account
Their Metabolism in the Human Body
A. V. Rudik
a,
*, A. V. Dmitriev
a
, A. A. Lagunin
a, b
, S. M. Ivanov
a, b
, D. A. Filimonov
a
, and V. V. Poroikov
a
a
Institute of Biomedical Chemistry, ul. Pogodinskaya 10, Moscow, 119121 Russia
b
Medico-Biological Faculty, Pirogov Russian National Research Medical University (RNRMU),
ul. Ostrovityanova 1, Moscow, 117997 Russia
*e-mail: rudik_anastassia@mail.ru
Received January 18, 2019; revised March 18, 2019; accepted March 18, 2019
Abstract—Most xenobiotics undergo metabolic conversions in the human body. The biological activity, tox-
icity, and other properties of such metabolites may significantly differ from those of the parent compounds.
Not only xenobiotics and their final metabolites produced in large quantities, but the intermediates and final
metabolites formed in trace amounts, can cause undesirable effects. We have developed a freely available web
application MetaTox (http://www.way2drug.com/mg/) for integral assessment of xenobiotics toxicity taking
into account their metabolism in humans. The generation of the metabolite structures is based on the reaction
fragments. The probability estimation of the certain reaction and the probability estimation of the atoms,
which are changed during biotransformation, are used for generation of the xenobiotic metabolism pathways.
The MetaTox web application assesses metabolism of compounds in humans and evaluates their acute toxic-
ity, specific (cardiotoxicity, hepatotoxicity, nephrotoxicity), and chronic toxicity (carcinogenicity, teratoge-
nicity, mutagenicity, effects on the reproductive system).
Keywords: biotransformation, metabolism, prediction, toxicity, PASS, MetaTox web application
DOI: 10.1134/S1990750819030065
INTRODUCTION
Most xenobiotics, which include pharmaceutical
substances, food additives, cosmetics, substances of
plant origin, industrial ecotoxicants, etc., undergo
biotransformation, involving various enzymes; this is
one of the most important mechanisms of the detoxi-
fication protective process, which mainly occurs in the
liver. Biotransformation of xenobiotics can include
several stages, thus forming a metabolic pathway for a
particular compound. In a normally functioning liver,
two types of biotransformation reactions take place;
these are usually classified as phase I and phase II
reactions [1]. During phase I reactions hydrophobic
molecules are transformed into more polar, hydro-
philic metabolites, which are more easily excreted by
the excretory system via oxidation, reduction or
hydrolysis [2]. Typical and most common enzymes
involved in phase I metabolism are enzymes from the
family of cytochromes P450, catalyzing oxidation of
xenobiotics. Phase II reactions of biotransformation
(also known as conjugation phase) involve various
transferases; the most common form of conjugation of
exogenous compounds is the reaction of glucuronide
formation catalyzed by UDP-glucuronyl transferases.
Conjugates are also more polar and more soluble in
water than parent substances and therefore they are
more readily excreted from the body.
Although in most cases the biotransformation pro-
cess results in formation of less active metabolites,
there is evidence for formation of xenobiotic metabo-
lites exhibiting higher toxicity [3] or reactivity [4].
Since not only xenobiotics and their final metabolites,
formed in large quantities, but also intermediate and
final metabolites, formed in trace amounts, may
exhibit toxic effects, evaluation of xenobiotic toxicity,
taking into account their metabolism in the human
body, is an important task for basic research in medi-
cine and toxicology.
Preclinical studies aimed at determination of
metabolites formed during biotransformation of drug
candidate compounds for analysis of their potential
toxic effects, include both animal experiments in vivo
and in vitro studies employing various cells and tissues
and animal organs [5].
However, such biotransformation studies are asso-
ciated with certain difficulties, since the metabolic
transformations of xenobiotics in experimental ani-
mals may be completely different from their biotrans-
formation in the human body [6]. Therefore, there is a
clear need in development of computerized prediction
methods applicable for evaluation of pharmacokinet-