PHYSICAL REVIEW C 109, L041604 (2024)
Letter
Longitudinal ternary fission
G. Royer ,
*
A. Aguilera, and V. Fasquel
Subatech Laboratory, UMR: IN2P3/CNRS-Université-IMT, 44307 Nantes, France
(Received 24 February 2024; accepted 28 March 2024; published 15 April 2024)
The longitudinal ternary fission is studied using the generalized liquid drop model. The proximity energy and
the charge and mass asymmetries are taken into account. Spherical parent and daughter nuclei are considered.
The shape sequence selected to simulate the quasimolecular three-body shapes is built from different but
connected elliptic half lemniscatoids. The potential barriers are much lower when the central fragment is the
smallest one and particularly when it is an α particle. The 2α emission can be described as a particular prolate
fission with emission of two particles at the tips of the deformed nucleus. The associated potential barriers are
high and thin.
DOI: 10.1103/PhysRevC.109.L041604
Ternary fission is a very rare nuclear decay mode but it
has been observed in several experiments at low energy [1,2]
or in heavy-ion reactions [3–5]. The third particle is mainly
an α particle. In the reaction with
36
Ar beams on a
24
Mg
target at high angular momentum, narrow correlations have
been interpreted as a ternary fission from an elongated shape,
the lighter mass in the neck region consisting of one, two,
or even three α particles with very low momentum in the
center-of-mass frame [6]. α particles emitted at rest in the
breakup of
28
Si into the
12
C +α +
12
C moleculelike configura-
tion have also been observed [7]. Another example is the true
ternary fission of
252
Cf leading to
132
Sn +
48,50
Ca +
70,72
Ni in
collinear geometry [8]. For general decays it has been shown
that the formation of the lightest fragment at the center has
the highest probability [9]. It has also been proved that the
potential barriers of the oblate ternary fission are higher than
the ones of the prolate ternary fission except perhaps for the
superheavy nuclei [5,10].
Theoretically, the ternary fission has been investigated stat-
ically and dynamically, assuming mainly specific shapes and
the formation in the neck of a third light particle which stays
almost at rest between the two other fragments which go away
[11–20].
The next question is now to study the possibility for a nu-
cleus to emit simultaneously two α particles. An experiment
has been proposed at CERN to investigate the double-α decay
from a nucleus. Theoretically, recently [21] a model for the
description of the simultaneous emission of two α particles
from the opposite sides of the nucleus has been discussed
in detail for nuclei with Z < 95. It uses analytical nuclear
and Coulomb potentials. Within a modified generalized liquid
drop model [22] the 2α decay has been studied in the re-
gion 93 < Z < 102 [23]. A microscopic theoretical approach
based on relativistic energy density functionals has also been
*
royer@subatech.in2p3.fr
used to compute axially symmetric deformation energy sur-
faces as functions of quadrupole, octupole, and hexadecupole
collective coordinates [24]. It is focused on
216−220
Rn and
220−224
Ra.
The purpose of this work is to determine the potential
barriers of the path leading a nucleus to emit one particle at
each tip of the initial nucleus within the generalized liquid
drop model [25] and selected shapes [26]. To study the fusion
and binary fission through compact and creviced shapes, a
shape sequence was defined [25] using two halves of different
lemniscatoids joined by a same radius of the neck (see Fig. 1).
In polar coordinates this shape is given by
R(θ )
2
=
a
2
sin
2
θ + c
1
2
cos
2
θ 0 θ π/2,
a
2
sin
2
θ + c
2
2
cos
2
θ π/2 θ π,
(1)
where a is the transverse distance and the radius of the neck
when there is a crevice, while c
1
and c
2
are the elongations
along the axis of revolution.
To simulate the longitudinal ternary fission with the small-
est fragment in the middle [14], a symmetry plane was
introduced cutting one fragment along its maximal orthogonal
distance (see Fig. 2). The same shape sequence can be used
when the central fragment is the biggest one, the two nuclei
at the extremes being identical. In particular, this allows us to
describe the simultaneous emission of two α particles at the
two opposite tips of the fissioning parent nucleus (see Figs. 3
and 4). Such a true ternary fission is very different from the
formation of a small nucleus in the neck between nascent
fragments.
Mathematically (Fig. 5), the two dimensionless parameters
s
1
= a/c
1
and s
2
= a/c
2
completely define the shape, with
a being the neck radius. The shape sequence evolves from a
sphere when s
1
= s
2
= 1 to three aligned spherical fragments
in contact when s
1
= s
2
= 0. For a given reaction with an
emission of a central fragment of radius R
2
and of two other
external identical fragments of radius R
1
, the parameters s
1
2469-9985/2024/109(4)/L041604(5) L041604-1 ©2024 American Physical Society