Vol.1, No.2, 77-85 (2010)
doi:10.4236/jbpc.2010.12010
Copyright © 2010 SciRes. Openly accessible at http://www.scirp.org/journal/JBPC/
Journal of Biophysical Chemistry
Distance-dependent coherent charge transport in DNA:
crossover from tunneling to free propagation
Natallia V. Grib
1*
, Dmitry A. Ryndyk
2
, Rafael Gutiérrez
3
, Gianaurelio Cuniberti
3
1
Department of Micro- and Nanoelectronics, Belarusian State University of Informatics and Radioelectronics, Minsk, Belarus;
*Corresponding Author: ngrib@uvic.ca
2
Institute for Theoretical Physics, University of Regensburg, Regensburg, Germany
3
Institute for Material Science and Max Bergmann Center for Biomaterials, Dresden University of Technology, Dresden, Germany
Received 8 June 2010; revised 4 July 2010; accepted 10 July 2010.
ABSTRACT
Using a tight-binding model, we investigate the
influence of intra- and interstand coupling pa-
rameters on the charge transport properties in a
G-(T)
j
-GGG DNA sequence and its (G:C)-(T:A)
j
-
(G:C)
3
duplex attached to four electrodes. De-
pendences of the transmission function and of
the corresponding conductance of the system
on the number of bridging sites were obtained.
Simulation results of a recently proposed two-
strand superexchange (tunneling) model were
reproduced and extended. It is demonstrated
that the crossover from strong to weak dis-
tance-dependent charge transport is elucidated
by a transition from under-barrier tunneling
mechanism to free over-barrier propagation in
the coherent regime, controlled by temperature
and coupling parameters. The role of DNA-
electrode coupling has been also considered. It
was found that an asymmetry in the DNA-elec-
trode coupling has a drastic effect on the con-
ductance leading to an increase in delocaliza-
tion of the electronic states in the DNA duplex.
Keywords: DNA; Electron Transport; Modeling of
DNA; Electronic Structure of DNA
1. INTRODUCTION
The discovery of charge migration in deoxyribonucleic
acid (DNA) stimulated intensive investigations of the
electronic properties of DNA due to their significance in
biosynthesis and radiation-induced damage and repair
processes [1-3]. Furthermore, considerable interest in
nanodimensional structures of DNA possessing unique
self-assembling and self-recognition properties has in-
creased the last decade in connection with the possibility
of the development of molecular nanoelectronic devices
which are expected to provide high storage of informa-
tion and high-speed signal processing within a wide
temperature range [4-6]. In fact, DNA molecules can be
well combined with silicon technology transcending the
potential of the present quantum wires and are supposed
to be used in modern computer technology as a binary
data structure by applying a programmable linear self-
assembly of the sequence of complementary nucleic
base pairs of DNA [7,8].
Until now numerous experimental and theoretical data
on charge migration through DNA molecules show an
apparently contradictory behavior which can be eluci-
dated by supposing two primary mechanisms. They in-
clude the single-step superexchange (tunneling) charge
transfer that is strongly dependent on length of a mo-
lecular chain, and the multi-step hopping mechanism
that is characterized by a weak change in the charge
transfer efficiency (CTE) with increasing of the donor-
acceptor distance in the double helix [9-11]. However,
experimental measurements of DNA molecule do not
give any unequivocal evidence in favor of one or other
mechanism of charge transfer in DNA. Many of them
demonstrate a combined hopping-superexchange mech-
anism with a transition from the coherent superexchange
to the thermally induced incoherent hopping process.
Beside electron transfer experiments, also transport
experiments became an important field of modern re-
search. In transport measurements a molecule is placed
between metallic leads and steady-state current can be
produced by finite voltage. A direct measurement of
electrical transport through single biological molecules,
such as DNA and peptides [12,13], is a very appealing,
although challenging, issue in molecular electronics be-
cause of the potential peculiar capabilities of forming self-
assembled nanodevices at the molecular scale. Quantum
transport experiments through single DNA oligomers
This work was funded by the Deutsche Forschungsgemeinschaft (SPP
1243) and Collaborative Research Center SFB 689.