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Speciation and preconcentration of vanadium(V) and
vanadium(IV) in water samples by flow injection-inductively
coupled plasma optical emission spectrometry and ultrasonic
nebulization
Rodolfo G. Wuilloud,
a
Jorgelina C. Wuilloud
a
Roberto A. Olsina
ab
and Luis D.
Martinez*
ab
a
Department of Analytical Chemistry, Faculty of Chemistry, Biochemistry and Pharmacy,
National University of San Luis, Chacabuco and Pedernera, P.O. Box 375, 5700 San Luis,
Argentina
b
Consejo Nacional de Investigaciones Científicas y Técnicas (CONICET), Argentina
Received 4th December 2000, Accepted 14th March 2001
First published as an Advance Article on the web 24th April 2001
An on-line separation, preconcentration and determination system for vanadium(IV) and vanadium(V) comprising
inductively coupled plasma optical emission spectrometry (ICP-OES) coupled to a flow injection (FI) method with
an ultrasonic nebulization (USN) system was studied. The vanadium species were retained on an Amberlite
XAD-7 resin as a vanadium–2-(5-bromo-2-pyridylazo)-5-diethylaminophenol (V–5-Br-PADAP) complex at
pH 3.7. Enhanced selectivity was obtained with the combined use of the formation on-line of the complexes and
1,2-cyclohexanediaminetetraacetic acid (CDTA) as masking agent. The vanadium complexes were removed from
the microcolumn with 25% v/v nitric acid. A sensitivity enhancement factor of 225 was obtained with respect to
ICP-OES using pneumatic nebulization (15-fold for USN and 15-fold for the microcolumn). The detection limit
for the preconcentration of 10 mL of aqueous solution was 19 ng L
21
. The precision for 10 replicate
determinations at the 5 mg L
21
V level was 2.3% relative standard deviation (RSD), calculated from the peak
heights obtained. The calibration graph using the separation and preconcentration system for vanadium species
was linear with a correlation coefficient of 0.9992 at levels from near the detection limits up to at least 100 mg
L
21
. The method was successfully applied to the speciation of vanadium in river water samples.
Introduction
The chemical and physical properties of a metal species depend
very much on its oxidation state, hence an accurate determina-
tion of each species is important for evaluating both the
potential risk and benefits of some metals.
1,2
Vanadium has
various oxidation states and ionic forms in aqueous solution. It
exists in two different oxidation states, V(V) and V(IV), in well
aerated natural and industrial waters.
3,4
The significance of
vanadium speciation is that the two oxidation states have
different nutritional and toxic properties.
5,6
The toxicity of V is
dependent on its oxidation state, with V(V) being more toxic
than V(IV).
3
Otherwise, the insulin-like properties of V,
especially its effects on mitogenesis, suggest that the element
plays a role in growth and development.
5
Therefore, the
speciation and determination of V are receiving increasing
attention in pollution and nutritional studies.
Since one of the routes of incorporation of V into the human
body is water,
6–8
its determination in this type of sample is very
important. The concentration of V in natural water is very
low,
9–11
of the order of a few mg L
21
, hence powerful
techniques are required and only a few of them show sufficient
sensitivity. Neutron activation analysis (NAA)
12,13
has been
applied to the determination of V, but it is time consuming and
the routine analysis of numerous samples is laborious. This
method also requires sophisticated instrumentation which may
not be available in most analytical laboratories. Inductively
coupled plasma mass spectrometry (ICP-MS)
14,15
is used for
the determination of V because of its high sensitivity, high
selectivity and high sample throughput. However, the cost of
the instrumentation may be prohibitive to many laboratories.
Inductively coupled plasma optical emission spectrometry
(ICP-OES) or electrothermal atomic absorption spectrometry
(ETAAS) are the most commonly used techniques for the
determination of traces of V, but the low level of V
concentration in water is not compatible with the detection
limits of these techniques. In order to achieve accurate, reliable
and sensitive results, preconcentrations and separations are
needed when the concentrations of the analyte elements in the
sample are too low to be determined directly by ICP-OES.
Many separation and preconcentration techniques
6,16,17
for
the determination of V(V) and V(IV) species have been
proposed, including chelation and extraction, precipitation and
the use of ion-exchange resins. However, many of these
methodologies are performed in batch, thus requiring large
sample volumes in order to reach low detection limits. Further,
these systems have higher contamination risks and are not
practical for application in routine analysis. This situation has
been significantly improved by utilizing flow injection (FI)
associated with ICP-OES.
18,19
In fact, to date the most dramatic
improvements achieved in FI-ICP-OES have been in the field of
on-line preconcentration.
20,21
On the other hand, the use of an
ultrasonic nebulizer can provide a 5–50-fold improvement in
detection limits.
22–24
XAD resins have been used as packing materials in
preconcentration columns for FI.
25,26
They have been employed
as supports for the immobilisation of chelating agents and metal
complexes.
27–29
2-(5-Bromo-2-pyridylazo)-5-diethylamino-
phenol (5-Br-PADAP) forms stable complexes with numerous
metal ions,
30,31
and is therefore a suitable reagent for V
preconcentration on an XAD resin.
32
Recently we have reported
a preconcentration FI system for the determination of total V
This journal is © The Royal Society of Chemistry 2001
DOI: 10.1039/b009705p Analyst, 2001, 126, 715–719 715