American Journal of Environmental Engineering 2013, 3(5): 207-212
DOI: 10.5923/j.ajee.20130305.02
Investigation of Factors Affecting THMs Formation in
Drinking Water
Motasem Saidan
1,*
, Khale d Rawajfe h
1
, Manar Fayyad
2
1
Chemical Engineering Department, University of Jordan, Jordan
2
Water Researches Center, University of Jordan, Jordan
Abstract Total Trihalomethanes (THMs) content can vary greatly, depending both on water quality and on treatment
conditions, in the same water supply system. Most municipal water treatment plants use chlorine to keep water biologically
safe during the distribution process. The effect of various parameters on the formation of THMs has been studied in this
investigation using water samples collected from Zai water treatment plant in Jordan. These parameters are reaction time,
temperature, pH, TOC, free chlorine, and bromide ion content. An increase in the value of any of these parameters has
positive effects on the formation of THMs. A general correlation for the prediction of THMs as a function of these parameters
is proposed. Its predictions are in good agreement with the observed results regardless of the fact that it is restricted to this
study. The kinetics of THMs formation were also investigated and found to follow first order kinetics with 0.0022 hr
-1
rate
constant.
Keywords THMs Formation, Chlorination, Drinking Water, Water Quality Model
1. Introduction
Chlorine, while an effective disinfectant, reacts with
organic materials that might be present in the source drinking
water to produce a group of chlorinated organic compounds
known as Disinfection Byproducts (DBPs)[1, 2]. The DBPs
include THMS (chloroform, bromodichloromethane,
dibromochloromethane, and bromoform). The presence of
THMs in drinking water has been the subject of increasing
public concern since the 1970s[3]. Toxicological studies
suggested that THMs have been linked to the occurrence of
human cancer in many instances in 1976. This was soon
followed by an act by the Environmental Protection agency
(EPA) to regulate their concentrations in drinking water.
In the past, various investigations had been conducted to
determine factors that might influence THMs formation[4].
From the mid of 1980s, several models simulating the
propagation and transformation of contaminants in a
distribution system over time were developed and applied
[5, 6]. In spite of water treatment, finished water may sustain
substantial changes in quality while being transmitted
through the distribution system before reaching the
consumer’s tap. These changes may be associated with
complex physical, chemical and biological processes that
take place during transport.
* Corresponding author:
m.saidan@gmail.com (Motasem Saidan)
Published online on October 26th 2013 at http://journal.sapub.org/ajee
Copyright © 2013 Scientific & Academic Publishing. All Rights Reserved
Statistical correlations has been developed to predict the
concentration of chloroform formation as function of pH,
temperature and distance (near or far) between a reservoir
and a point of interest in the distribution system. This
correlation is qualitative in the sense that distance and time
are not included implicitly in it[7].
Multiple regression model has been generated for
predicting THMs level in the finished water leaving a
treatment plant. The correlation implies that THMs
formation is higher in summer through autumn and lower in
winter through spring[8].
Mathematical model that applies second order kinetics has
been proposed to predict the chlorine residuals and
demonstrates that THMs formation can be characterized as a
function of chlorine demand. The parameters of this model
are correlated as a function of pH, TOC, temperature and
chlorine residual[9].
The formation of THMs in drinking water has been shown
to be a function of various water quality parameters and
chlorination conditions. THMs formation is one of the
slowest known reactions in water treatment and a number of
important factors influence this reaction. These include
residence time, pH, temperature, bromide ion concentration,
chlorine dosage, type of organic precursor and the Total
Organic Carbon (TOC).
In the present paper, the overall objective is to develop an
improved understanding of the effect of water parameters on
THMs formation in drinking water, and also develop a
mathematical model for the prediction of THMs
concentrations for Zai water treatment plant.