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INVESTIGATION ON N-FORMYL PIPERIDIN-4-ONES AS CORROSION INHIBITORS
FOR CARBON STEEL IN ACID MEDIUM
A. ILAMPARITHI
1
, S. PONNUSWAMY
2
& A. SELVARAJ
3
1,2
PG and Research Department of Chemistry, Government Arts College (Autonomous), Coimbatore, Tamil Nadu, India
1
Department of Chemistry, Gobi Arts and Science College, Gobichettipalayam, Tamil Nadu, India
3
PG and Research Department of Chemistry, CBM College, Coimbatore, Tamil Nadu, India
ABSTRACT
The corrosion inhibition of mild steel in 1N H
2
SO
4
and 1N HCl in the presence of N-formyl piperidin-4-ones was
studied using gravimetric and electrochemical techniques. Results obtained show that these compounds are excellent
inhibitors and inhibit better in HCl than in H
2
SO
4
. The potentiodynamic polarisation studies clearly reveal that they are
mixed type inhibitors. The impedance parameters (R
ct
and C
dl
) clearly indicate the adsorption of N-formyl piperidin-4-ones
on the metal surface leading to the formation of a protective layer which grows with increasing exposure time.
The adsorption of N-formyl derivatives on mild steel surface in both the acid media follows a Langmuir adsorption
isotherm and Tempkin adsorption isotherm. The mild steel-FP complex layer formed at the metal surface was identified by
infrared spectral analysis and SEM/EDS.
KEYWORDS: 1. Corrosion Inhibitors, 2. Mild Steel, 3. Electrochemical Impedance Spectroscopy, 4. Polarisation
Curves, 5. Adsorption Isotherm, 6. N-Formyl Piperidin-4-One, 7. FT-IR , 8. SEM/EDS
INTRODUCTION
Generally HCl and H
2
SO
4
are employed in the treatment of steel and ferrous alloys in industry. The use of
inhibitors containing heteroatom’s like nitrogen, oxygen, and sulphur is one of the most practical methods for protection
against corrosion in acid media
[1]
. The aim of this study is to investigate the inhibitive properties of some azacyclic
inhibitors viz. N-formyl-t-3-methyl-r-2,c-6-diphenylpiperidin-4-one (F3MPO), N-formyl-t-3-isopropyl-r-2,
c-6-diphenylpiperidin-4-one (F3IPPO), N-formyl c-3,t-3-dimethyl-r-2,c-6-diphenylpiperidin-4-one (F3DMPO) and
N-formyl t-3,c-5-dimethyl-r-2,c-6-diphenylpiperidin-4-one (FDMPO) on the corrosion of mild steel in sulphuric acid and
hydrochloric acid. The chemical structures of the inhibitors are given in Figure 1.
(A) (B)
International Journal of Applied and
Natural Sciences (IJANS)
ISSN(P): 2319-4014; ISSN(E): 2319-4022
Vol. 3, Issue 2, Mar 2014, 63-80
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