INVESTIGATING THE EFFECT OF VULCANIZATION IN TREAD RUBBER
APPLICATIONS
Jatinder Kumar
1,a
and Rupinder Singh
2,b
1.
Dept. of Mechanical Engineering, ARNI University, Kathgarh-Indora, Distt- Kangra, H.P., India
2.
Dept. of Production Engineering, Guru Nanak Dev Engineering College, Ludhiana, Punjab, India
a
Er_jatinderkumar@yahoo.com,
b
rupindersingh78@yahoo.com
Keywords: Tread, vulcanization, retreading, strength, elongation, hardness, curing temperature.
Abstract. Retreading has many potential applications in tyre manufacturing industry. There is a
critical need for optimization of ‘vulcanization processes used in tread manufacturing. Not much
work hitherto has been reported for optimization of efficient sulphur vulcanization process of the
tread manufacturing. The present experimentation work highlights approach to macro-model
strength, elongation and hardness during vulcanization of rubber. Relationship between strength,
elongation, hardness and other parameter has been deduced by using Taguchi L9 orthogonal array
(OA). Results indicate that the hardness, elongation and strength of tread rubber while vulcanization
depends significantly on the ‘natural: synthetic rubber ratio’ (NR: SR), ‘curing time’ and ‘curing
temperature’ of the rubber.
Intorduction
Vulcanization is a chemical process for converting rubber or related polymers into more durable
materials via the addition of sulphur or other equivalent chemical known as “curatives" [1]. These
additives modify the polymer by forming cross-links between individual polymer chains. The
vulcanized material is less sticky and has superior mechanical properties [5]. The un-vulcanized
natural rubber is sticky, easily deforms when warm, and is brittle when cold. In this state it cannot
be used to make articles with a good level of elasticity [2]. The reason for inelastic deformation of
un-vulcanized rubber is due to its chemical structure: rubber is composed of long polymer chains.
These chains can move independently relative to each other, which enables the material to change
shape [4]. The cross linking introduced by vulcanization prevents the polymer chains from moving
independently. As a result, when stress is applied the vulcanized rubber will deform, but upon
release of the stress, the material will revert to its original shape. Kok [2] examined the effect of
compounding ingredients on the reversion of accelerated sulphur vulcanization of NR. Accelerators
which normally provide fast cures are found to cause more severe reversion than slower
accelerators. MgCO3, CaCO3, silica and china clay all increase reversion but the severity depends
on the accelerated system employed. Mukhopadhyay et al. [9] investigated the effect of
vulcanization temperature (150°–180°C) on the structure and technical properties of NR
vulcanizates with four different accelerator {2-(morpholinodithio)-benzothiazole} : sulphur ratios
(A - 0.6:2.4, B-1.5:1.5; C - 2.4:0.6; D-3.0:0.0) at the respective optimum cure times. The influence
of cure temperature on the chemical crosslink density was determined. Results show that elevated
cure temperatures produce a network with lower crosslink density. Kuriakose and Rajendran [1]
proposed the use of raw rice bran oil in the vulcanization of carbon black and silica filled systems in
NR compounding in place of process oil, antioxidant and fatty acid and concluded that results are
not much affecting the cure characteristics of the mixes and physical properties of the vulcanizates.
Apart from the low cost of the product, it will be helpful in also saving energy during mixing. The
high free fatty acid content and non-toxic nature of this non-edible natural oil could therefore be an
added advantage in the rubber product manufacturing industry[11]. Ismail and Chia [3] investigated
the concentration effects of multifunctional additive (MFA) and vulcanization systems on silica
filled epoxidized natural rubber (ENR 25) in the concentration range 0–7.5 phr. Three vulcanization
systems were used; conventional vulcanization (CV), semi-efficient vulcanization (semi-EV) and
efficient vulcanization (EV). The cure time and scorch time of all vulcanization systems decrease
Materials Science Forum Vol. 751 (2013) pp 1-7
© (2013) Trans Tech Publications, Switzerland
doi:10.4028/www.scientific.net/MSF.751.1
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