Jointly published by React.Kinet.Catal.Lett.
Akadémiai Kiadó, Budapest Vol. 82, No. 2, 255-261
and Kluwer Academic Publishers, Dordrecht (2004)
0133-1736/2004/US$ 20.00.
© Akadémiai Kiadó, Budapest.
All rights reserved.
RKCL4417
AMPHIPHILIC NaY ZEOLITE PARTICLES LOADED WITH NIOBIC
ACID: MATERIALS WITH APPLICATIONS FOR CATALYSIS IN
IMMISCIBLE LIQUID-LIQUID SYSTEM
Hadi Nur
a*
, Shigeru Ikeda
b
and Bunsho Ohtani
b
a
Ibnu Sina Institute for Fundamental Science Studies, Universiti Teknologi Malaysia, 81310
UTM Skudai, Johor, Malaysia
b
Catalysis Research Center, Hokkaido University, Sapporo 060-0811, Japan
Received September 24, 2003
In revised form December 18, 2003
Accepted January 23, 2004
Abstract
The catalytic potential of catalysts for acid-catalyzed reactions has been
demonstrated by NaY zeolite loaded with alkylsilane-covered niobic acid in the
liquid phase hydration of 1,2-epoxyoctane with water. The catalytic activity of
the catalysts was correlated to the amphiphilic character of the solid catalyst
particles.
Keywords: Amphiphilic zeolite particles, acid-catalyzed reactions
INTRODUCTION
The fast-growing insight into green chemistry has led to research more
focused on the area of environmentally benign catalysts [1, 2]. Along this line,
we recently reported a new approach to modify the surface of zeolite, resulting
hydrophilic and hydrophobic regions, for application as catalyst in immiscible
liquid-liquid systems in co-solvent free condition [3-6]. The organic
transformations under solvent-free conditions are attracting increasing
attention because the use of large quantities of organic solvents is not only
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*Corresponding author. E-mail: hadi@kimia.fs.utm.my