Parveen Sulthana et al. 1
© 400
Terminalia chebula Retz. gallic acid – biased silver nanoparticles and
their antiphytopathogenic activity
A. Parveen Sulthana
1
, J. Martin Rathi
2*
and K. Sahayaraj
3
ABSTRACT
Owing to the unique properties, nanomaterials play a major role in many areas of science and
technology. In this paper the antiphytopathogenic activity of gallic acid reduced Terminalia chebula
Retz. silver nanoparticles (Ag NPs) was studied. AgNO
3
(10
-3
M) stock solution was prepared by
dissolving 17mg of silver nitrate in 100ml of double distilled water. 10ml of gallic acid solution
isolated from Terminalia chebula Retz. (Combretaceae) was added to 90ml of 10
-3
M AgNO
3
solution for reduction of Ag
+
ions. The reduction of pure Ag
+
ions was monitored by measuring in
the UV-Vis Spectroscopy at 426nm. Determination of the shape and structure of silver nanoparticle
was characterized by Transmission Electron Microscopic (TEM) and X-ray Diffraction studies
(XRD). The plasma resonance of the gallic acid reduced silver particle is brownish yellow. In the
light of these studies, the shape of the silver nanoparticle (spherical) and face centered cubic (FCC)
structure were explained. The antibiotic experiment conducted in the present study revealed the
antiphytopathogenic activity of gallic acid reduced Terminalia chebula Retz. silver nanoparticles
against the phytopathogen Xanthomonos axonopodis pv. malvacearum and also confirmed the
antiphytopathogenic activity studies based on “Broth microdilution method” against Xanthomonos
axonopodis pv. malvacearum.
MS History: 05.11.2013 (Received)-05.03.2014 (Revised)-17.03.2014 (Accepted)
Key words: Terminalia chebula, gallic acid, silver nanoparticles, TEM, XRD, antiphytopathogenic activity.
INTRODUCTION
Silver has been in use since time immemorial in the
form of metallic silver, silver nitrate, silver
sulfadiazine for the treatment of burns, wounds and
several bacterial infections (Mahendra Rai et al.,
2009). But due to the emergence of several
antibiotics, the use of these silver compounds has
declined remarkably. However silver nanoparticles
could be used as a potential alternative therapy to
reduce severity of disease due to Pseudomonas
aeruginosa infections (Navindra Kumari
Palanisamy et al., 2014). Nanotechnology is gaining
tremendous impetus in the present century due to its
capability to modulate metals into their nanosize,
which drastically changes their chemical, physical
and optical properties. Hence metallic silver in the
form of silver nanoparticles has made a remarkable
comeback as a potential antimicrobial agent. The
use of silver nanoparticles is also important, as
several pathogenic bacteria have developed
resistance against various antibiotics. It has diverse
medical applications ranging from silver based
dressings, silver coated medicinal devices, such as
nanogels (Mahendra Rai et al., 2009), nanolotions
(Mahendra Rai et al., 2009) etc. The nanocrystalline
silver dressings, creams and gel effectively reduce
bacterial infections in chronic wounds (Richard et
al., 2002; Leaper, 2006; Ip et al., 2006). Silver
impregnated medical devices like surgical masks
and implantable devices show significant
antimicrobial efficacy (Furno et al., 2004). There
are numerous works related to green synthesis of
metallic nanoparticles using higher plants. Gardea-
Toroesday et al., (2003) first reported the formation
of silver nanoparticles by living plants. Shankar et
al. (2004) reported pure metallic silver nanoparticles
synthesis by the reduction of Ag
+
and Au
+
ions
using neem (Azadirachta indica Juss.) leaf broth.
For instance, some of the renowed reports on
phytosynthesis of silver nanoparticles by employing
lemon grass extract ( Shankar et al., 2004, 2005),
green tea, Camellia sinensis (L.) Kuntze (Vilchis-
Nestor et al.,2008), Aloe vera (L.) Burm. Plant
extract (Chandran et al., 2006), sundried
Nanoparticles antiphytopathogenic activity JBiopest 7(Supp.): 1-6 (2014)