Knowledge of Research 2014, 1(1), 62-67
Research Article
DOI:10.7598/kor2014.106
Naema A. Hikmat
*
,
Ahlam M. Farhan
2
and
Rana Afif Majed
3
1
Chemistry Department,
College of Science,
Baghdad University, Iraq
2
Chemistry Department,
College of Science for Woman,
Baghdad University, Iraq
3
Materials Engineering Department,
University of Technology, Iraq
dr.rana_afif@yahoo.com
Received 3 November 2014
Revised 13 November 2014
Accepted 10 November 2014
©ISSAC Publications
http://www.knowledgeofresearch.com
Thermodynamic and Kinetic
Parameters for Corrosion Inhibition
of Al-Cu alloy by Sodium Acetate
at pH 11
Abstract: Corrosion inhibition properties of Al-Cu alloy in 0.001 M
NaOH solution at pH 11 were investigated at four temperatures
include 298, 303, 308 and 313 K using potentiostat by adding
sodium acetate as inhibitor with three concentrations 0.05, 0.1 and
0.15 M. Corrosion parameters, protection efficiencies,
thermodynamic and kinetic functions have been measured to
estimate the inhibition efficiency of Al alloy in experimental
conditions. The results indicate that 0.05 M of sodium acetate is
the best concentration through the data of protection efficiency
which supported by the highest value of enthalpy. The values of
activation energy became higher indicating the inhibitive action
of acetate. The entropy of activation values was negative.
Keywords: Al-Cu alloy, Sodium acetate, Corrosion inhibition.
Introduction
Aluminium alloys are widely employed within the spacecraft industry and they provide the required
mechanical and corrosion properties. The choice of Al-alloy depending on its application, the 2xxx series
(high copper content) and 7xxx series (high zinc content) are used for structural components due to their
high toughness and good fatigue strength. Generally these alloys offer a good corrosion resistance for most
environmental exposures. However specific environmental conditions, such as long period storage in humid
and salty environments, may trigger corrosion and therefore these alloys require additional protection.
An earlier works reported that copper reduces the pitting initiation resistance of aluminium and
therefore it was advised to add small quantities of copper (up to 0.15%) to aluminium in order to reduce the
pits depths by other increasing pits density
1,2
. On the other hand Galvele and Micheli
3
and Muller and
Galvele
4
studied the effect of copper on breakdown potential E
b
value for aluminium in different
concentrations of NaCl solutions and on both (1M NaCl) and saturated AlCl
3
solutions respectively. They
found that the presence of copper in solid solution in aluminium shifts E
b
to more noble values; however this
beneficial effect is limited by the solubility of copper in aluminium.
The effect of copper to the preferential dissolution of aluminium from the attacked region attribute to Cu
– enrichment inside the pits which can reduce the cathodic reaction over potential. The later result was
supported by Bicelli et al.
5
who studied the effect of copper on E
b
value for aluminium in 3.5% NaCl
solution. They found that E
b
value for Al–Cu alloy in the solution treated condition followed by natural
ageing was slightly above that for commercially pure aluminium (99.9% Al). Recently, many authors
interested corrosion behavior and protection of Al-Cu alloy in different media
6-11
.