International Research Journal of Engineering and Technology (IRJET) e-ISSN: 2395 -0056
Volume: 02 Issue: 02 | May-2015 w.irjet.net p-ISSN: 2395-0072
© 2015, IRJET.NET- All Rights Reserved Page 442
Modification of Sorghum Starch for Production of Superabsorbents
M. D. Teli
1
, A. Mallick
2
1
Professor of Fibres and Textile Processing, Dept. of Fibres and Textile Processing Technology, Institute of Chemical
Technology, Maharashtra, India
2
Ph.D. Tech. Research Scholar, Dept. of Fibres and Textile Processing Technology, Institute of Chemical Technology,
Maharashtra, India
Abstract - Starch extracted from Sorghum bicolor
grains was gelatinized and grafted with acrylic acid
(AA) and acrylamide (AAm) using potassium
persulphate(KPS) as an initiator. Different parameters
of grafting reaction such as reaction time, temperature,
initiator concentration, and starch to monomers ratio
were optimized. Material thus produced was dried,
grounded and characterized using FT-IR and SEM.
Grafted starch products were saponified with 0.1 N
NaOH solution followed by neutralization and drying.
Maximum absorbency of 225.5 gg
-1
in normal water was
obtained, qualifying it as super absorbent product
(SAP).
Keywords: Grafting, Starch, Superabsorbent
1. INTRODUCTION
Superabsorbent polymers are hydrophilic polymers which
are able to absorb and retain a fairly large amount of water
within their structure. This becomes possible as the
polymers, which are hydrophilic in nature, do not get
dissolved in water and hold the water molecules within
their swollen three dimensional interconnected structures
(hydrogels). There is no definite lower limit of absorbency
to call a hydrogel as a superabsorbent, and many authors
have referred their hydrogels with high absorbency as
superabsorbent when the water retention capacity of the
polymer was more than 100 times of its own dry weight
(or more than 1000%)[1]. These hydrogels attracted wide
interest due to their intriguing properties such as high
absorption and swelling capacity, slow release of moisture,
etc. Some of these products are widely used in personal
care, agriculture and biomedical applications [2].
Although synthetic superabsorbent polymers show very
high water retention properties and fair to good gel
strength, the biodegradability of these acrylate based SAPs
is very poor causing increase in environmental load [3].
Therefore, incorporation of biopolymers for synthesis of
SAP became preferred option to the use of their synthetic
counterparts. Products made of natural biopolymers are
biodegradable and more importantly, their sources are
cheap, renewable and sustainable.
Natural biopolymers such as cellulose, starch, etc. are
effective alternative of synthetic superabsorbent polymers
[4,5]. Starch is basically composed of two fractions,
amylopectin and amylose and both constitute 97-98% of
dry weight of starch. These are polysachharides and their
ratio varies with the botanical origin of the starch. Great
Millet or Sorghum (Sorghum bicolor L.Moench) is a cheap
and alternative source of starch. Sorghum, commonly
known as jowar in )ndia is the world’s fourth major cereal
in terms of production, and fifth in acreage following
wheat, rice, maize and barley, and serves as a staple food
crop in India [6. Sorghum grain contains starch ranging
from 68-75% depending upon variation in seed quality,
region and climatic conditions [7].
Grafting of starch has been widely reported by different
researchers. Different polymerization techniques viz.
solution polymerization, emulsion polymerization,
suspension polymerization, polymerization via irradiation,
etc. are used for producing superabsorbent hydrogels.
Different initiation systems such as ceric ammonium
nitrate, potassium persulphate etc. also have been used for
these processes [8,9]. Chen et al. (2004) utilized batata
starch for grafting with acrylic acid and acrylamide under
gamma radiation with polyethylene glycol as crosslinker
[10]. Cassava starch has been grafted by acrylamide using
ceric ammonium nitrate by Jyothi et al. (2012) [3]. Peng et
al (2007) on other hand used acrylamide (AAm),
diallydimethylammonium chloride (DMDAAC) and sodium
starch sulfate for producing SAP using ammonium
persulpfate as grafting initiator [2].
The present paper deals with extraction of starch from
sorghum and its modification as a superabsorbent by
grafting hydrophilic monomers onto it. It discusses the
optimization of the process as well as the characterization
of the modified starch and the product developed as a
superabsorbent.