Silyl Derivatization of Alkylphenols, Chlorophenols,
and Bisphenol A for Simultaneous GC/MS
Determination
Donghao Li and Jongman Park*
Department of Chemistry, Konkuk University, 1 Hwayangdong Gwangjingu, Seoul 143-701, Korea
Jae-Ryoung Oh
Korea Ocean Research and Development Institute, Ansan P.O. Box 29, Gyounggido 425-600, Korea
A fast silyl derivatization technique for simultaneous GC/
MS analysis of alkylphenols, chlorophenols, and bis-
phenol A was developed. The analytes were silylized with
an excess amount of bis(trimethylsilyl)trifluoroacetamide
(BSTFA) followed by hydrolysis of excess silyl reagent with
water. Reaction rates of derivatization were studied in
various solvents and found to be fastest in acetone.
Derivatization reaction in acetone was completed quan-
titatively within 1 5 s at room temperature while it took
more than 1 h in other solvents studied. Similar results
were obtained in mixed solvents with acetone if the
content of acetone was higher than 6 0 % (v/ v). Since water-
immiscible solvents such as dichloromethane or hexane
are frequently used in the extraction of phenolic analytes
in various sample matrixes, acetone can be added to the
extracts in order to accelerate the reaction rate of deriva-
tization. Stability of the derivatives in sample for long-term
storage was ensured by hydrolyzing excess derivatizing
reagent, BSTFA, with a spike of water followed by dehy-
dration using anhydrous sodium sulfate. On the basis of
the above results, a derivatizing treatment kit was de-
signed to improve the convenience of analysis. It was
possible to treat sample within several minutes success-
fully by using the kit. So fast simultaneous determination
of those anlaytes by GC/ MS was possible with improved
convenience as well as sensitivity and reproducibility.
Alkylphenol ethoxylates (APEs), chlorophenols (CPs), and
bisphenol A (BPA) have been widely used in the preparation of
detergents, wood preservatives, and polymeric materials for
household and industrial applications. They have been discharged
directly or indirectly to the environment and contaminated the
atmosphere, water, and soil. APEs are degraded to alkylphenols
(APs) during an aerobic or anaerobic waste treatment process or
by microorganism
1
and photolysis
2
in nature. Although the APEs
are less toxic to organisms, their metabolites
3,4
show high toxicity
to organisms and fish.
5,6
So most countries have classified them
as endocrine disrupter chemicals.
7-11
Numerous papers have been
published about determination of APs, CPs, and BPA using various
techniques. Some of the most frequently used methods for
analysis of these are as follows: direct analysis using HPLC,
12-14
GC/ ECD,
15-17
LC/ MS,
18
GC/ MS,
19,20
and other techniques
21,22
or
indirect analysis of the compounds using derivatization techniques
such as methylation,
23
acetylation,
24,25
and silylation.
26-28
Methyl-
ation and acetylation techniques are suitable for the analytes
* To whom correspondence should be addressed: (phone) +82-2-450-3438;
(fax) +82-3436-5382; (e-mail) jmpark@ kkucc.konkuk.ac.kr.
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Anal. Chem. 2001, 73, 3089-3095
10.1021/ac001494l CCC: $20.00 © 2001 American Chemical Society Analytical Chemistry, Vol. 73, No. 13, July 1, 2001 3089
Published on Web 05/16/2001