Coordination Networks with Flexible Ligands Based on Silver(I) Salts:
Complexes of 1,3-Bis(phenylthio)propane with Silver(I) Salts of PF
6
-
,
CF
3
COO
-
, CF
3
CF
2
COO
-
, CF
3
CF
2
CF
2
COO
-
, p-TsO
-
, and CF
3
SO
3
-
Mohamed Osman Awaleh, Antonella Badia, and Franc ¸ ois Brisse*
De ´ partement de chimie, UniVersite ´ de Montre ´ al, C.P. 6128, Succursale Centre-Ville,
Que ´ bec, Canada H3C 3J7
Received April 21, 2005
The synthesis and characterization of nine coordination networks based on 1,3-bis(phenylthio)propane, L
3
, and
silver(I) salts of PF
6
-
(1), CF
3
COO
-
(2), CF
3
CF
2
COO
-
(3), CF
3
CF
2
CF
2
COO
-
(4), p-TsO
-
(5, 6), and CF
3
SO
3
-
(7-9) are reported. Only 1 and other “isostructural” complexes with weakly coordinating anions such as ClO
4
-
and
SbF
6
-
are of the host-guest type. In all the other complexes, the anions and the acetone molecules, when present,
are coordinated to the metal. Most of the complexes studied here form a 2D-coordination network. Only 4 and 5
adopt a polymer-like chain structure. The packing of the chains of 4 is pseudohexagonal compact, while that of 5
is of the centered type. In complex 1, the silver atom is tetrahedrally coordinated to the sulfur atoms of four
different ligands. The PF
6
-
anions and acetone molecules, sandwiched between silver-ligand cationic sheets, are
held through van der Waals interactions. In each of the three perfluorocarboxylates (2-4), two silver atoms are
joined by the anions in a diatomic bridging mode. The Ag‚‚‚Ag distances are sufficiently short to indicate weak
metal‚‚‚metal interactions. The dimeric units in 2 and 3 are interconnected through the ligands, thereby generating
a 2D-network of neutral sheets, while, in 4, the dimeric units are bound to four ligands and a 1D-coordination
polymer is generated. In the case of the sulfonate anions (p-TsO
-
and CF
3
SO
3
-
), the crystallization solvent influences
the structure adopted. Thus, in 5, 7, and 9 obtained from petroleum ether, or other nonpolar solvents, two silver
atoms are bound in a double-bridge fashion, while a monobridge mode is noted for 6 and 8, both recrystallized
from diethyl ether. In 8, both bridging types are observed. The thermogravimetric investigation, in the room
temperature-450 °C interval, of complexes 1, 3, and 7, which incorporate acetone molecules in their crystal structures,
reveals a two-step weight loss for 1 (the acetone molecules are lost first followed by the ligands, leaving behind
the silver salt), while complexes 3 and 7 decompose in a single step to metallic silver.
Introduction
In the last two decades, there has been considerable activity
in the design and synthesis of solid frameworks.
1
The self-
assembly of metal-organic coordination polymers has at-
tracted a great deal of attention because of their potential
applications as functional materials.
2
The properties of
coordination polymer materials are to some extent dependent
on their network topology. Thus, it is of interest to understand
and control the subtle factors that influence the formation
of these supramolecular networks. Moreover, the strategy
consisting of varying the coordination site and/or the size
and shape of the ligand is usually employed in crystal
engineering to synthesize new coordination polymers. The
metal centers are linked with rigid bridging ligands
3
or less
frequently by flexible building blocks.
4
However, for a given
* To whom correspondence should be addressed. E-mail: francois.brisse@
umontreal.ca. Fax: (+)-(514) 343-7586.
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Inorg. Chem. 2005, 44, 7833-7845
10.1021/ic050617n CCC: $30.25 © 2005 American Chemical Society Inorganic Chemistry, Vol. 44, No. 22, 2005 7833
Published on Web 09/30/2005