ISSN 1063-7842, Technical Physics, 2008, Vol. 53, No. 8, pp. 1065–1069. © Pleiades Publishing, Ltd., 2008.
Original Russian Text © V.A. Krivchenko, D.V. Lopaev, P.V. Pashchenko, V.G. Pirogov, A.T. Rakhimov, N.V. Suetin, A.S. Trifonov, 2008, published in Zhurnal Tekhnicheskoœ Fiziki,
2008, Vol. 78, No. 8, pp. 107–111.
1065
INTRODUCTION
Zinc oxide (ZnO) is a wide-band semiconductor
with a bandgap roughly equal to 3.3 eV [1]. This fact,
combined with a high binding energy of excitons at
room temperature, renders this material promising for
UV light-emitting diodes [2–4]. As applied to solar-
blinded (UV) photodetectors [5–7] and gas sensors [8],
the main advantages of ZnO over other materials are its
transparency in the visible range, high thermal stability,
and high chemical inertness [9].
A number of efficient UV detectors based on single-
crystalline ZnO [6], polycrystalline ZnO films [5], and
nanocrystalline ZnO films [7] have been described in
the literature to date. It was reported, for example, that
application of high-purity single-crystalline ZnO
allows designers to raise the efficiency of UV detectors
to 61%; however, such a technology is expensive,
related devices are limited in size, and tailor-made sub-
strates are required. In the case of nanocrystalline ZnO
films, the maximal efficiency of the detectors, 18%,
was reached in a multilayer p(20-nm-thick NiO)–i(200-
nm-thick ZnO)–n(50-nm-thick ITO) structure grown
on a glass substrate [7]. The disadvantage of such struc-
tures is that they, as a rule, are prone to degradation
because of chemical reactions at the interfaces. Photo-
detectors based on polycrystalline ZnO also show a
high quantum efficiency (44.9%) [5]. However, their
fabrication requires sapphire substrates, multistage
ZnO evaporation, and heat treatment of the substrate.
This all may considerably complicate the fabrication
technology of the detectors.
In this work, we study a simpler and more stable
design of UV detectors based on nanocrystalline ZnO
films. The films were deposited by magnetron sputter-
ing in an rf discharge. Our goal was to see how the type
of sputtered target and ZnO film deposition conditions
influence the photoelectric performance of the UV
detectors. In addition, we studied the efficiency of the
detector versus its surface topology, which was exam-
ined with an atomic force microscope (AFM).
EXPERIMENTAL
ZnO films were deposited on glass plates with pre-
applied contacts. The contacts were applied by magne-
tron sputtering of Ti (50 nm) and Au (50 nm) layers and
patterned by photolithography. We used an interdigi-
tated structure of electrodes (contacts) with spacings of
10 and 20 μm (Figs. 1a, 1b). Then, the contacts were
covered by 2-μm-thick ZnO films applied by magne-
UV Detectors Based on Nanocrystalline ZnO Films
V. A. Krivchenko, D. V. Lopaev, P. V. Pashchenko, V. G. Pirogov,
A. T. Rakhimov, N. V. Suetin, and A. S. Trifonov
Research Institute of Nuclear Physics, Moscow State University, Moscow, 119992 Russia
e-mail: victi81@mail.ru
Received August 20, 2007
Abstract—Nanocrystalline films of zinc oxide deposited by rf magnetron sputtering are used as a working
material of UV detectors. The photoelectric performance of UV detectors versus ZnO deposition conditions is
studied. The influence of the surface topology of the UV detectors on their efficiency is examined with an
atomic force microscope.
PACS numbers: 72.80.Ey, 73.40.Sx, 73.50.Pz, 73.63.Bd
DOI: 10.1134/S1063784208080148
OPTICS,
QUANTUM ELECTRONICS
(a)
(b)
(c)
(d)
300–600 nm
0–30 V
10
20
ZnO film
Gold contacts
ZnO film
Au contacts
Glass substrate
A
Fig. 1. (a, b) Optical microscopic images of the substrates
used in the experiment, (c) circuit used in measuring the
photoelectric properties of the UV detectors, and (d) cross-
sectional view of the UV detector (not to scale).
Amplifier