Polarization fields in the positronium atom undergoing emission or absorption of optical photons O. N. Gadomski and S. G. Moiseev Ul’yanovsk State University, 432700 Ul’yanovsk, Russia Submitted 20 March 1997 Zh. E ´ ksp. Teor. Fiz. 113, 471–488 February 1998 This paper solves the problem of the interaction of an electron and positron via the field of soft and hard photons with emission or absorption of a real photon. The interaction is interpreted as a third-order QED effect in the coordinate representation. The role of intermediate states with positive and negative frequencies is studied. A general expression is derived for the matrix elements of the operator of the effective electron–positron interaction energy for different types of quantum transitions. The expression makes it possible to calculate the probabilities of the corresponding transitions in the nonrelativistic approximation. Electric dipole transitions in the positronium atom accompanied by emission absorptionof an optical photon are investigated. Two-particle wave functions of the positronium atom are used to introduce the concept of polarization fields inside the positronium atom. It is found that the polarization fields depend on the coordinates and time and on the choice of the pair of states between which a quantum transition with emission or absorption of a photon takes place. © 1998 American Institute of Physics. S1063-77619800602-7 1. INTRODUCTION Polarization fields play an important role in shaping vari- ous optical processes. For instance, in the classical optics of insulators such a polarization field is the electric dipole field, 1 which allows not only for an explaination of reflection and refraction of light but also makes it possible to derive in a rigorous manner the Lorenz–Lorentz formula for the re- fractive index. As shown in Refs. 2 and 3, establishing the nature of polarization fields in insulators requires using an approach based on QED first- and second-order effects. This makes it possible to study various types of quantum transi- tion in the field of virtual and real photons and to allow for the orbital and spin degrees of freedom of the atomic elec- trons, the various types of intermediate states in the spectrum of interacting atoms, and the retardation effect for atoms lo- cated at arbitrary distances from one another. A considerable achievement here is the development of a method for obtain- ing new types of integral equations that describe the propa- gation of photons in a medium with allowance for different quantum-transition types electric dipole, quadrupole, mag- netic dipole, spin, etc.in the spectrum of atoms. 4,5 Here allowance is made for electron and positron polarization fields, which correspond to intermediate states of the atoms with positive and negative energies, respectively. An integral field equation in the electric dipole approximation has been used to study the laws of reflection and refraction of light in quantum 6 and nonlinear 4 optics, to build a theory of a non- linear refractive index, 4 and to theoretically predict the near- field effect with allowance for a discrete distribution of the atoms near the the observation point. 4,7 . In contrast to Refs. 1–7, our paper studies the role of polarization fields inside an individual atom. Drake 8 examined the interaction of two atomic electrons in a helium-like atom as a QED third-order effect. It was found that with allowance for the orbital and spin degrees of freedom and intermediate states with positive and negative energies, third-order effects lead only to relativistic correc- tions to the photon emission and absorption probability. The present paper is devoted to the theory of quantum transitions between the levels of the positronium atom in- duced by soft optical or radio-frequencyphotons. The need for such a theory derives from the use of precision methods of radio and optical spectroscopy in the physics of the posi- tronium atom, research into the annihilation process in highly excited states, 9–11 and the study of the possibility of markedly changing the kinetic characteristics of the annihi- lation process in the field of an optical laser. 12 . Obviously, the interaction of the positronium atom and the photon field is largely determined by the coupling constants in the effec- tive Hamiltonian. Hence we pay special attention to these constants by interpreting the optical transition between the levels of the positronium atom as a QED third-order effect. We find that these effects explain the one-photon processes of emission and absorption in the positronium atom due to the Coulomb electron–positron interaction and induced po- larization fields. We also find that calculations of the prob- ability per unit timeof spontaneous photon emission yield the same result if we use the single-particle wave functions of the positronium atom of Refs. 10 and 13 or the two- particle wave functions derived in the present paper. In other words, thanks to the specific properties of the positronium atom, third-order effects are most evident in such an atom, in contrast to the case of helium-like atoms. 8 As noted earlier, in this paper we use the two-particle wave functions of the positronium atom. First, this makes it possible to study the various schemes of quantum transitions JOURNAL OF EXPERIMENTAL AND THEORETICAL PHYSICS VOLUME 86, NUMBER 2 FEBRUARY 1998 259 1063-7761/98/86(2)/11/$15.00 © 1998 American Institute of Physics