© by PSP Volume 23 – No 12a. 2014 Fresenius Environmental Bulletin
3140
EFFECT OF ZEOLITE AND HALLOYSITE
ON ACCUMULATION OF TRACE ELEMENTS IN
MAIZE (Zea Mays L.) IN NICKEL CONTAMINATED SOIL
Maja Radziemska
1
, Zbigniew Mazur
2
, Joanna Fronczyk
1
, and Jerzy Jeznach
1,
*
1
Warsaw University of Life Sciences - SGGW, Faculty of Civil and Environmental Engineering, Nowoursynowska 159, 02-773 Warsaw, Poland
2
University of Warmia and Mazury in Olsztyn, Poland, Faculty of Environmental Management and Agriculture, Pl. Łódzki 4, 10-727, Olsztyn, Poland
Presented at the 17
th
International Symposium on Environmental Pollution and its
Impact on Life in the Mediterranean Region (MESAEP), September28 - October 01, 2013, Istanbul, Turkey
ABSTRACT
Plants grown in contaminated areas may accumulate
toxic levels of trace elements in their biomass. A pot
experiment was conducted to study the effects of increas-
ing nickel contamination on the accumulation of selected
trace elements in maize (Zea mays L.) after the applica-
tion of zeolite, raw and modified halloysite. In a vegeta-
tive-pot experiment, five different level of Ni contamina-
tion, i.e., 0 (control), 80, 160, 240, 320 mg·kg
–1
were ap-
plied in an analytical grade NiSO
4
.
7H
2
O solution mixed
thoroughly with the soil. The content of nickel, lead, zinc,
chromium, copper and manganese in maize depended on
the dose of nickel and type of neutralizing substance. The
average accumulation of trace elements in maize grown in
nickel contaminated soil were found to follow the decreas-
ing order nickel>zinc>manganese>copper>lead>chromium,
respectively. The highest reduction in nickel content was
observed in the above-ground parts of maize at sites
where 240 mg of Ni was used per 1 kg of soil following
the addition of zeolite and modified halloysite. The high-
est increase in chromium content was observed in the
above-ground parts of maize after row halloysite was
applied.
KEYWORDS: zeolite, halloysite, heavy metals, soil contamina-
tion, maize (Zea mays L.)
1. INTRODUCTION
The progressive degradation of soils with heavy met-
als is becoming one of the most severe environmental and
* Corresponding author
human health hazards. Moreover, people are especially at
risk, as contaminants present throughout the environment
accumulate in the human body. In small concentrations,
nickel is essential in facilitating the metabolism of calci-
um, zinc, iron, and hematopoiesis processes in the human
body [1]. It is one of the most mobile and bioavailable
heavy metal ions that may be present in soils. The forms
of Ni in soil containing minerals are pentlandite ((Fe,
Ni)
9
S
8
), cohenite ((Fe,Ni)
3
C), awaruite (Ni
3
Fe) and haxo-
nite ((Fe,Ni)
23
C
6
). Phytotoxicity caused by the contamina-
tion of the environment with nickel has recently received
increasing attention. The contamination of the environ-
ment with nickel compounds, modifies not only the phys-
icochemical properties of soil, but also negatively affects
plants [2, 3].
The application of low cost, easily available materials
in the removal of heavy metals from polluted soils has
been widely investigated. Zeolite is known to be a good
adsorbent for heavy metals, such as chromium, lead,
cadmium, copper, zinc and nickel [4, 5, 6]. The structures
of zeolites consist of three-dimensional frameworks of
SiO
4
and AlO
4
tetrahedra. Halloysite is a two-layered
aluminosilicate clay mineral with a natural nanotubular
structure, consisting of one alumina octahedron sheet and
one silica tetrahedron sheet in a 1:1 stoichiometric ratio.
Each of these two layers is separated by a monolayer of
interlayer water molecules [7]. It is chemically similar to
kaolin, differing mainly in the morphology of crystals.
This mineral is abundant in Poland as well as other areas
of the world. Halloysite has a large range of applications
in many fields, and is mainly used to produce high quality
porcelain products as an additive to polymer filters and in
plastics and other comparable composites.
The aim of the conducted research was to determine
the effect of soil contamination with nickel on the content
of microelement in the above-ground parts of maize (Zea
mays L.) and to examine whether the applied neutralizing
substances (zeolite, raw and modified halloysite) can be
effective in reducing their impact on crops.