Desalination 199 (2006) 390–392
Presented at EUROMEMBRANE 2006, 24–28 September 2006, Giardini Naxos, Italy.
Role of physico-chemical and hydrodynamic
aspects in cleaning of spiral PES ultrafiltration membranes
of dairy industry
Murielle Rabiller-Baudry*, David Delaunay, Lydie Paugam,
Lilian Bégoin, Bernard Chaufer
Chimie et Ingénierie des Procédés, UMR 6226 CNRS “Sciences Chimiques de Rennes”
Université Rennes 1– ENSCR, 263 avenue du général Leclerc, Campus Beaulieu Batiment 10 A,
CS 74205, 35042 Rennes cedex, France
email: murielle.rabiller-baudry@univ-rennes1.fr
Received 17 October 2005; accepted 1 March 2006
1. Introduction
Ultrafiltration (UF) of skimmed milk is
widely used in order to control the protein
content before the cheese making process. At
industrial scale, UF is generally performed
with spiral wound membranes of low cut-off
(typically 5–10 kg mol
–1
) made of polyether-
sulfone (PES). After water rinsing, an irre-
versible fouling remained. Consequently,
chemical cleaning is needed in order to
restore the flux. At industrial scale, the step of
cleaning (and further disinfection) is daily
performed via cleaning in place (CIP) sta-
tions, running in empirical and non-optimised
conditions and, finally, the recovered flux is
lower than that of the virgin membrane. As a
consequence, a progressive decrease of flux
during UF of dairy fluids is observed over fol-
lowing months of production. The general
cleaning scheme was performed at 50°C in
two steps: first an alkaline solution at pH =
11.5 known to be efficient toward organic
matter and then a cleaning with an acid solu-
tion at pH = 1.6 to remove mineral matter. As
the main target of cleaning is protein, the gen-
eral scheme of cleaning/disinfection can be
reduced to a single alkaline step limiting thus
water consumption for rinsing and produced
volume of effluents. The flux is not always
reliable as it can be modified independently of
the cleaning efficiency by adsorption of com-
ponents (surfactants, nitrates) of the cleaning
solution. In this context, the aim of this study
is first to propose physico-chemical parame-
ters to have an access to the effective cleaning
efficiency, to identify parameters governing
the cleaning and propose a guide to formulate
an adapted and optimised alkaline cleaning
solution. Two physico-chemical criteria were
proposed: the first is based on the quantifica-
tion of irreversible fouling, by FTIR-ATR,
directly on the membrane and the second on
interfacial energy of detergents. The cleaning *Corresponding author.
doi:10.1016/j.desal.2006.03.210
0011-9164/06/$– See front matter © 2006 Published by Elsevier B.V.