©
2013 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim 1 wileyonlinelibrary.com
COMMUNICATION
www.MaterialsViews.com
www.advopticalmat.de
A bidispersed magnetic colloid containing micrometer-sized
magnetizable spheres and nanomagnetic particles is an inter-
esting as well as intriguing scattering medium.
[1–3]
Optical wave
propagation in strongly scattering media or in partially ordered
systems exhibit several novel and useful phenomena. Strong
and weak localization, photonic Hall effects, and anisotropic dif-
fusion coefficients are some examples.
[4–6]
The most fascinating
phenomenon amongst these is that of the storage and retrieval
of light.
[7–9]
Successful attempts were also made to transport the
stored light some distance:
[10]
Scully and his group have trapped
laser signals (with help of a writer pulse) in ultra-cold rubidium
atoms10. Then the writer laser was switched off. After a frac-
tion of millisecond, another reader laser was switched on which
was at a distance of 6 millimeters away from the writer laser,
and the signal pulse was received. We demonstrate here a new
technique which is comparatively simpler, cost effective, and
which operates at room temperature.
In most of the above examples, scatterers were nonmagnetic
particles surrounded by a nonmagnetic medium. When scat-
terers are magnetic or the surrounding medium is magnetically
active, they exhibit new photonic effects.
[11–14]
When both the
scatterers as well as the medium are magnetizable, the system
manifests several intriguing possibilities. We show here that
such a scattering system can transport the stored light some
distance. Previously, we showed that such a ferrodispersion
exhibits several magnetically tunable photonic effects like weak
localization, zero scattering, photonic bandgaps, optical capaci-
tors, etc.
[15–19]
The most intriguing effect is the trapping and
release of light with the help of an externally applied magnetic
field.
[15]
The experiment was performed with the following con-
figuration: linearly polarized light was allowed to pass through
a diluted sample of magnetizable micrometer-sized spheres
(MMS). The latter was subjected to a static magnetic field. It
was observed that when the direction of propagation and the
electric vector of the incident light are transverse to the direc-
tion of the applied field, the emergent light from the sample
disappears at a critical value of the magnetic field. The light
reappears when the field is slightly more or less than this
value. The system was then subjected to the critical field and
was exposed to the incident light for some time and then the
light shutter was closed. Under this condition, the field was
switched off. Almost immediately, a flash of light with the same
frequency and state of polarization as that of the incident
light was observed. The findings were attributed to the trap-
ping of light at the critical field and its release when the field
was removed. The details of these findings are described else-
where.
[15]
In the present work, we show that the trapped light
can be carried some distance and retrieved at this distance. We
have also studied the role of the size of the MMS, the wave-
length of incident light, and the exposure time, and results are
analyzed in terms of morphology-dependent resonance (MDR)
induced by the applied magnetic field.
Methods of preparation of stable suspensions of micrometer-
sized magnetite particles and the ferrofluid are described in
earlier papers.
[13,16]
Commercially available magnetite powder
was first washed with dilute nitric acid to remove impurities.
The powder was then washed with double-distilled water and
acetone. The dried powder was mixed with kerosene and ball-
milled in the presence of oleic acid. Using fractional sedimen-
tation, suspensions containing 1, 2, and 3 μm-sized particles
were obtained. The particles were found to be almost spherical.
Ferrofluid was synthesized by co-precipitating nanomagnetic
particles of magnetite and coating these particles with oleic
acid. Again kerosene was used as a base liquid. Aggregation, if
any, was removed by centrifuging the fluid at 12 000 rpm. The
average particle size of the nanomagnetic particles was deter-
mined using X-ray diffraction and was found to be ∼10 nm.
Saturation magnetization of the fluid was 200 Gauss. Each sus-
pension of MMS was mixed with the ferrofluid and diluted with
kerosene as per the requirement. These samples were homog-
enized by ultrasonification and no sedimentation was observed
during the experimental measurements. The sample under
investigation was poured into a rectangular glass cell with
a 2 mm path length. All the samples were found to be trans-
parent at this path length.
The schematic of the experimental setup is shown in
Figure 1 a. A 5 mW diode pumped solid state (DPSS) green
laser ( λ = 532 nm) and a He–Ne 10 mW laser ( λ = 632 μm)
were used as light sources. A Glan–Thomson polarizing prism
was used to convert unpolarized light into polarized light and
the axis of the polarizer was arranged so that E-vector of the
light incident on the glass cell remained perpendicular to the
direction of the applied field. An electromagnet was driven
by a constant current power supply. The magnetic field was
measured using a Hall probe. The rectangular cell filled with
the ferrodispersion was fixed between the pole pieces of the
magnet and was mounted on an x-y-z platform, and its posi-
tion could be read by a micrometer screw. The translation of the
stage in the direction of the magnetic field was controlled by a
motor. Emerging light from the sample was detected by a CCD
camera. This camera was also mounted on a translation stage.
Provision was made to introduce another glass cell of 1 cm path DOI: 10.1002/adom.201300123
Experimental Demonstration of Magnetic Carriage for
Transport of Light Trapped in Magnetizable Mie Spheres
Rajesh Patel, and Rasbindu V. Mehta*
Prof. R. Patel, Prof. R. V. Mehta
Department of Physics
Maharaja Krishnakumarsinhji Bhavnagar University
Bhavnagar, 364002, India
E-mail: rvm@bhavuni.edu
Adv. Optical Mater. 2013,
DOI: 10.1002/adom.201300123