Retention of Ionizable Compounds on HPLC. 12.
The Properties of Liquid Chromatography Buffers
in Acetonitrile -Water Mobile Phases That
Influence HPLC Retention
Sonia Espinosa, Elisabeth Bosch, and Martı´ Rose ´s*
Departament de Quı ´ mica Analı ´ tica, Universitat de Barcelona, Diagonal 647, E-08028 Barcelona, Spain
The addition of acetonitrile to aqueous buffers to prepare
RP HPLC mobile phases changes the buffer properties
(pH and buffer capacity). This variation is studied for ace-
tate, phosphate, phthalate, citrate, and ammonia buffers
in acetonitrile-water mixtures up to 6 0 % in acetonitrile
(v/ v). Equations are proposed to relate pH and buffer
capacity change of these buffers to the initial aqueous pH
value and to the volume fraction of acetonitrile added. It
is demonstrated that the pH change of the buffer depends
not only on the initial aqueous pH of the buffer and on
the percentage of acetonitrile added but also on the
particular buffer used. The proposed equations allow an
accurate prediction of this ionization for the studied
buffers. Since the retention of acid/ base compounds
shows a strong dependence of their degree of ionization,
the equations are used to predict the change in this
ionization with addition of acetonitrile when the RP HPLC
mobile phase is prepared. This prediction allows estima-
tion of the retention of an acid/ base compound in a
particular acetonitrile-water buffered mobile phase.
Buffers are widely used for pH control of chemical processes.
1
In reversed-phase high-performance liquid chromatography (RP
HPLC) separations of compounds with acid/ base properties,
appropriate buffered solutions are needed for calibration of the
electrode system used to measure pH and for control of the
mobile-phase pH, since the latter influences analyte ionization and
thus retention.
pH standardization of electrode systems in water and in the
most used RP HPLC mobile phases has been substantially
achieved. The IUPAC has endorsed rules for pH standardization
in water and in water-organic solvent mixtures of moderate to
high permittivities and proposed some buffered solutions for pH
standardization in these solvents.
2-4
Some additional buffers in
acetonitrile-water have been studied by Barbosa et al.
5-7
On the
basis of IUPAC rules and recommendations, we have studied the
different pH scales that are employed in pH measurement of RP
HPLC mobile phases. Three different pH scales have been used.
The most common is the aqueous pH scale (
w
w
pH), which is
obtained when the electrode system is calibrated with aqueous
buffers and the pH measured in the RP HPLC aqueous buffer
before mixing it with the organic modifier. If the electrode system
is calibrated with aqueous buffers, but the pH is measured in the
mobile phase obtained after mixing the aqueous buffers with the
organic modifier, the pH scale in the mobile-phase solvent (s)
relative to water (w) as standard-state solvent is obtained (
w
s
pH).
Finally, if the electrode system is calibrated with buffers prepared
in the same mixed solvent used as mobile phase (s) and the pH
is measured in the mobile phase (s), the pH scale in the mobile
phase referred to the same mobile phase as standard-state solvent
is obtained (
s
s
pH). Whenever possible, we recommend
s
s
pH and
w
s
pH scales because they give much better general relationships
between pH and retention.
8-10
The
w
s
pH scale is specially recom-
mended because of its simplicity of measurement, since it does
not require pH standards for each different mobile-phase composi-
tion.
However, the main acid/ base properties of the buffers used
to control the pH of RP HPLC mobile phases has not been
systematically studied. In a pioneer work, Bates discussed the
properties of acid/ base aqueous buffers and its applicability to
chemical processes.
1
Bates remarked that in choosing a suitable
buffer system, one should not only consider the pH required but
should also take into account the nature of the reaction to be
regulated. A high buffer capacity is essential for the control of an
acid/ base reaction, and a low dilution value is desirable if dilution
of the medium is likely to occur. The dilution value is defined as
the increase of pH suffered by a solution when it is diluted with
an equal volume of pure solvent. Salt effects and temperature
changes may be important in some instances. The chemical nature
* Corresponding author. Fax: 34 93 402 12 33. E-mail: marti@ apolo.
qui.ub.es.
(1) Bates, R. G. Determination of pH: Theory and Practice, 2nd ed.; Wiley: New
York, 1964.
(2) IUPAC Compendium of Analytical Nomenclature. Definitive Rules 1997, 3rd
ed.; Blackwell: Oxford, U.K., 1998.
(3) Mussini, T.; Covington, A. K.; Longhi, P.; Rondinini, S. Pure Appl. Chem.
1985 , 57, 865-876.
(4) Mussini, P. R.; Mussini, T.; Rondinini, S. Pure Appl. Chem. 1997 , 69, 1007-
1014.
(5) Barbosa, J.; Sanz-Nebot, V. Anal. Chim. Acta 1993 , 283, 320-325.
(6) Barbosa, J.; Butı ´, S.; Sanz-Nebot, V. Talanta 1994 , 41, 825-831.
(7) Barbosa, J.; Sanz-Nebot, V. Mikrochim. Acta 1994 , 116, 131-141.
(8) Canals, I.; Portal, J. A.; Bosch, E.; Rose ´s, M. Anal. Chem. 2000 , 72, 1802-
1809.
(9) Espinosa, S.; Bosch, E.; Rose ´s, M. Anal. Chem. 2000 , 72, 5193-5200.
(10) Canals, I.; Oumada, F. Z.; Rose ´s, M.; Bosch, E. J. Chromatogr., A 2001 ,
911, 191-202.
Anal. Chem. 2002, 74, 3809-3818
10.1021/ac020012y CCC: $22.00 © 2002 American Chemical Society Analytical Chemistry, Vol. 74, No. 15, August 1, 2002 3809
Published on Web 07/03/2002