Mass Spectrometry for
Clinical Toxicology:
Therapeutic Drug
Management and Trace
Element Analysis
Alan L. Rockwood, PhD, DABCC*, Kamisha L. Johnson-Davis, PhD, DABCC
KEYWORDS
• Mass spectrometry • Ionization • Toxicology
• Clinical chemistry • Therapeutic drug monitoring
• Therapeutic drug management
Mass spectrometry is rapidly expanding its role in clinical chemistry. To date, this
growth has primarily been in the area of small molecule analysis, though the field now
seems set for a rapid growth of protein and peptide analysis. Small molecule analysis
applications can be grouped roughly into the analysis of endogenous compounds and
the analysis of exogenous compounds. The analysis of exogenous compounds is
largely the domain of toxicology, and this is the focus of this article.
To limit the scope and, therefore, the length of this article, we focus primarily on 2
general topics within clinical toxicology: therapeutic drug monitoring and trace
element analysis. While these 2 topics do not cover the full breadth of mass
spectrometry applications in clinical toxicology, omitting, for example, clinical drugs-
of-abuse testing and applications supporting poison control programs, we feel that
they, nevertheless, provide a fairly representative overview of mass spectrometry in
the clinical toxicology lab.
TECHNOLOGY AND TECHNIQUE
As an aid to those readers who are less familiar with mass spectrometry technology,
we also provide a brief tutorial on the technology of mass spectrometry. This section
can also be read as an aid in understanding this article and other articles within this
volume.
Department of Pathology, University of Utah School of Medicine and ARUP Laboratories, 500
Chipeta Way, Salt Lake City, UT 84065, USA
* Corresponding author.
E-mail address: rockwoal@aruplab.com
Clin Lab Med 31 (2011) 407– 428
doi:10.1016/j.cll.2011.07.003 labmed.theclinics.com
0272-2712/11/$ – see front matter © 2011 Elsevier Inc. All rights reserved.