261
Mater. Res. Soc. Symp. Proc. Vol. 1538 © 2013 Materials Research Society
DOI: 1 557/op 013 0.1 l.2 .
Low-temperature Photoluminescence Studies of CdTe Thin Films Deposited on
CdS/ZnO/Glass Substrates
Corneliu Rotaru
1
, Sergiu Vatavu
1,2,3
, Christoph Merschjann
2
, Chris Ferekides
3
,
Vladimir Fedorov
1
, Tobias Tyborski
2
, Mihail Caraman
1
, Petru Gaúin
1
, Martha Ch. Lux-Steiner
2
and Marin Rusu
1,2
1
Faculty of Physics and Engineering, Moldova State University, 60 A. Mateevici str., MD-2009
Chisinau, Republic of Moldova
2
Institut für Heterogene Materialsysteme, Helmholtz-Zentrum Berlin für Materialien und
Energie, Lise-Meitner-Campus, Hahn-Meitner-Platz 1, 14109 Berlin, Germany
3
Department of Electrical Engineering, University of South Florida, 4202 East Fowler Ave,
Tampa, FL 33647, USA
ABSTRACT
The CdTe photoluminescence spectra of CdTe/CdS/ZnO heterojunctions annealed in the
presence of CdCl
2
have been analyzed in the 4.7-100K temperature range. The analysis has been
performed for laser excitation power between 0.01 mW and 30 mW. The analysis showed that
the photoluminescence spectrum in the 1.1-1.6 eV region consists of a defect band (1.437 eV)
having complex structure and revealing well contoured LO phonon replicas and bound exciton
annihilation in the 1.587-1.593 eV region. The band analysis has been carried out by
deconvoluting the spectra. It has been shown that the defect band consists of two elementary
bands and their phonon replica. An “unusual” temperature dependence of the defect band has
been found.
INTRODUCTION
CdTe-based thin film heterojunctions used for PV device fabrication continue to be a
promising means of direct solar to electricity conversion. Defects and dopants are important to
further enhancement of PV parameters. One of the possibilities to explore the direct
consequences of technology influence on the development of CdTe solar cells is thorough study
of the low-T photoluminescence (PL). This technique can reveal photo-active levels and can be
used to relate their influence to solar cell performance.
In particular, PL analysis is suitable for investigating the influence of the technology
variations during the fabrication of CdS/CdTe heterojunctions [1] for photovoltaic use. The
analysis publications related to the topic of investigation shows that the results and the
interpretation of the physical processes in CdTe related to luminescence differ and are sometimes
ambiguous. Such situations often occur when authors cross-reference to results measured in
different experimental set-ups (i.e. different excitation lasers, etc.) or to different samples
(annealed/unannealed, thin film or single crystal etc.).
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