Pressure of fluids and solids composed of particles interacting with a short-range repulsive potential Siegfried Hess 1 and Martin Kro ¨ ger 1,2 1 Institut fu ¨r Theoretische Physik, Technische Universita ¨t Berlin, PN 7 1, Hardenbergstrasse 36, D10623 Berlin, Germany 2 Polymer Physics, Department of Materials, ETH Zu ¨rich, ML H 18, CH-8092 Zu ¨rich, Switzerland Received 15 October 1999 A simple short range repulsive potential SR, with an even smoother cut off than the Weeks-Chandler- Andersen WCA–Lennard–Jones potential, yields practically the same pressure, both in the fluid state and for the fcc solid, when the potential parameters are chosen such that the forces are the same at the distance where the the two potential curves are equal to k B T . The comparison of the pressure for the SR and the WCA systems is based on molecular dynamics computer simulations. The fluid branch of the equation of state is rather well described by a modified Carnahan-Starling expression. PACS numbers: 47.10.+g, 62.10.+s, 64.10.+h, 66.20.+d INTRODUCTION A fluid composed of particles which interact via the 6-12 Lennard-Jones LJpotential cut off at its minimum and shifted such that it vanishes at the cut off distancewas con- sidered by Weeks, Chandler, and Andersen WCA1as a ‘‘hard-sphere-like’’ reference system. This interaction with a purely repulsive force is frequently referred to as the WCA potential. In Ref. 1, effects of the attractive force in a fluid with the full LJ interaction potential were treated as a per- turbation. Due to its short range of interaction and its smooth cut off, the WCA potential, taken as a model as such, is quite popular in equilibrium and nonequilibrium molecular dy- namics MD and NEMDcomputer simulation studies. It is the purpose of this note to point out that a computationally still simpler short range repulsive potential SR, with an even smoother cut off, yields practically the same pressure, both in the fluid state and in the fcc solid, provided that the forces are the same at the distance where the the two poten- tial curves are equal to k B T . The comparison of the pressure for the SR and the WCA systems is based on MD computer simulations. The fluid branch of the equation of state is rather well described by a modified Carnahan-Starling CS expression 2,3. I. THE POTENTIAL CURVES The Lennard-Jones LJpotential, cut off in its minimum at r cut and shifted such that it is zero at the cutoff distance r cut , was used by Weeks, Chandler, and Anderson 1as a purely repulsive reference potential. The WCA potential, for r r cLJ =2 1/6 r 0 1.122r 0 , is given by WCA r =4 0  r / r 0 -12 -r / r 0 -6 + 0 , 1 and WCA ( r ) =0 for r r cLJ . The quantities 0 and r 0 set the characteristic energy and length scales. A system com- posed of WCA particles possesses solid and fluid phases but no gas-liquid phase transition. The SR potential, introduced in Ref. 4, is defined by SR r = 0 9 -8 r / r 0 3 , r r csh = 9 8 r 0 =1.125r 0 , 2 and SR ( r ) =0 for r r csh . The potential parameters in Eq. 2have been chosen such that, at r =r 0 , the values of the potential functions and of their first derivatives are equal, viz., ( r 0 ) = 0 and ' ( r 0 ) =-24 0 / r 0 , for both poten- tials. In the following, results for the pressure are presented for the temperature T = 0 / k B . In a quantitative comparison of analytic calculations with results obtained by MD simulations for the structure of a ferrofluid, an equivalent scaling was used to relate a r -12 soft sphere potential to a screened Coulomb interaction 5. In numerical calculations and in the graph displayed here, all physical quantities are expressed in the standard LJ units of Refs. 6–9, e.g., lengths and energies are given in units of r 0 and 0 . When no danger of confusion exists, the dimen- sionless variables will be denoted by the same symbols as the original quantities. Then the WCA and SR potentials read WCA ( r ) =4( r -12 -r -6 ) +1, r r cLJ =2 1/6 , WCA ( r ) =0 for r r cLJ , and SR ( r ) =(9 -8 r ) 3 , r r csh =1.125, SR ( r ) =0 for r r csh . Similarly, the number density n =N / V , where N and V are the number of particles and the volume of the system, and the temperature T are expressed in units of n ref =r 0 -3 and T ref = 0 / k B , respectively. The unit for the pressure is p ref = 0 r 0 -3 . II. PRESSURE VERSUS DENSITY A. Remarks on MD simulations Simulations at the constant temperatures T / T ref =1 and constant number densities n =N / V ( NVT simulationsin the range n / n ref =0.1, . . . , 1.2 were performed for N =10 3 =1000 and 4 8 3 =2048 particles, where the initial posi- tions were simple cubic and face centered cubic fcclattice sites. The equations of motion were integrated with the ve- locity Verlet algorithm with the time step t / t ref =0.002. The LJ reference time is t ref =r 0 ( m / 0 ) (1/2) , and m is the mass of a particle. A cubic simulation box with volume V and peri- odic boundary conditions were used. The temperature was PHYSICAL REVIEW E APRIL 2000 VOLUME 61, NUMBER 4 PRE 61 1063-651X/2000/614/46293/$15.00 4629 © 2000 The American Physical Society For your personal use only. Not for redistribution related contributions available from the author(s) at www.complexfluids.ethz.ch