1 Copyright © 2011 by ASME
Proceedings of the ASME 2011 Internal Combustion Engine Division Fall Technical Conference
ICEF2011
October 2-5, 2011, Morgantown, West Virginia, USA
ICEF2011-60233
MODELING OF SCR NH
3
STORAGE IN THE PRESENCE OF H
2
O
Michael A. Smith
University of Michigan
Ann Arbor, MI, USA
Christopher D. Depcik
University of Kansas
Lawrence, KS, USA
John W. Hoard
University of Michigan
Ann Arbor, MI, USA
Stanislav V. Bohac
University of Michigan
Ann Arbor, MI, USA
Dionissios N. Assanis
University of Michigan
Ann Arbor, MI, USA
ABSTRACT
Diesel engines offer excellent fuel economy, but this
comes at the expense of higher emissions of nitrogen oxides
(NO
x
) and Particulate Matter (PM). To meet current emissions
standards, diesel engines require aftertreatment devices.
Concepts using combinations of catalysts are becoming more
common in aftertreatment systems to reduce the cost and size
of these aftertreatment systems. One combination is an LNT-
SCR system where the LNT releases NH
3
during a regeneration
to be used by the SCR catalyst for further NO
x
reduction. This
involves rich-lean cycling of the exhaust stream, which alters
species concentrations in the exhaust. Most notably H
2
O and
CO
2
levels can vary from 4% - 14% during lean-rich cycling.
An investigation was performed using multiple Temperature
Programmed Desorption (TPD) experiments to determine how
H
2
O and CO
2
affect NH
3
storage capacity of an Fe-based
zeolite SCR catalyst. It was determined that H
2
O and CO
2
inhibit NH
3
storage capacity of the SCR catalyst. This
inhibition has shown a linear dependence on H
2
O and CO
2
concentration at constant temperature. It was also determined
that H
2
O is a much stronger inhibitor of NH
3
storage capacity
then CO
2
. Additional Temperature Programmed Desorption
(TPD) experiments, were run where H
2
O and CO
2
concentration (0%, 6%, and 10%) and the initial storage
temperature (200°C, 250°C, 300°C, 350°C) were varied.
Results suggest the addition of a reaction that creates
competition for active sites on the catalyst between H
2
O and
NH
3
. The additional reaction allows H
2
O and NH
3
to be stored
on open catalytic sites and has improved model accuracy by
accounting for large changes in H
2
O, CO
2
, and temperature.
INTRODUCTION
Future emission regulations target dramatic reductions in
the levels of carbon monoxide (CO), hydrocarbons (HC),
nitrogen oxides (NO
x
) and particulate matter (PM) produced by
internal combustion power plants. For the traditional spark-
ignition engine, these problematic species are eliminated using
Close Coupled Catalysts (CCC) near the exhaust manifold and
underbody Three-Way Catalysts (TWC) in a system that
approaches 100% efficiency [1, 2]. However, for lean burn
engines, the choice is not as clear. The lean combustion
characteristics of these engines often force the OEM to utilize
multiple devices to convert all problematic species [3-5]. This
is because a singular device does not exist for diesel engines for
simultaneous conversion of CO, HC and NO
x
similar to a CCC
or TWC in spark-ignition engines. Current efforts at lowering
diesel NO
x
emission levels use retarded fuel injection and large
amounts of cooled Exhaust Gas Recirculation (EGR) to reduce
the in-cylinder combustion temperature [6, 7]. However, in-
cylinder techniques alone cannot reduce emission levels to
below regulatory standards [8].
Copper (Cu) and iron (Fe) are the two major types of
zeolite cations for SCR catalysts. Fe-zeolites have the largest
temperature operating range, while Cu-zeolites have lower
sensitivity to the NO:NO
2
ratio in the exhaust stream. Cu-
zeolites are also less susceptible to sulfur poisoning and have a
higher NH
3
storage capacity than Fe-zeolites [9, 10].
While zeolites do have promise, a major issue with respect
to SCR applications is the availability of NH
3
for conversion of
NO
x
. Instead of using an on-board Diesel Exhaust Fluid (DEF)
tank, it is possible to combine Lean NO
x
Trap (LNT) and SCR
catalysts, similar to the Eaton Aftertreatment System (EAS)
shown in Figure 1 [11, 12]. The LNT-SCR system uses the