International Journal of Engineering & Technology IJET-IJENS Vol: 11 No: 01 197
118401-5353 IJET-IJENS © February 2011 IJENS
I J E N S
A Photo-Cathodic Protection System Utilizing UV Radiations
Intesar Ahmed*, Zaki Ahmad**, Faheemuddin Patel**, M. Shuja Khan*
**Mechanical Engineering Department,
**King Fahd University of Petroleum & Minerals, Dhahran, Saudi Arabia
*Department of Electrical Engineering,
*COMSATS Institute of Information Technology, Lahore, Pakistan
Email: *drintesarahmad@ciitlahore.edu.pk , **ahmadz@kfupm.edu.sa
Abstract - Metallic corrosion of steel can be successfully
prevented by using a TiO
2
based photo-electrochemical system
under UV radiations. A TiO
2
semiconductor in a scavenging
medium (water or formate) generates photocurrent and shifts
the potential of steel to more negative values. This paper
describes a cathodic protection system using a TiO
2
photoanode.
The system has a potential to be developed for field applications
because it is capable of fulfilling the dual functions of both
cathodic protection as well as environmental cleaning.
Keywords: UV radiation, Photo-electrochemical
process, TiO
2
, C.B (Conduction Band).
1. INTRODUCTION
Corrosion is a major threat to the integrity of costly
hydrocarbon assets such as onshore and offshore plants,
transport pipelines, infrastructure and process systems and
its devastating regimes extending to critical assets, utilities
and buildings as well. Cathodic protection and coatings are
the two largest contributors to the direct cost of corrosion,
which shows the importance of these techniques to mitigate
corrosion. In cathodic protection, a substantial progress has
been made which is shown by the development of
computerized surveillance and mitigating techniques for
AC and DC couplings [1]. New anodes comprising of
conductive ceramic tubes or cylinders of metal matrix
oxide composites (MMC) coated with titanium solid in
mesh form are being produced. With the emergence of
nanotechnology and increasing demand on green
environment, investigations have been undertaken to study
the photocatalytic effect of titanium dioxide [2-5]. Photo-
electrochemical techniques of corrosion prevention of steel
and have been suggested [6-12]. Studies undertaken in
recent papers have shown that the cathodic protection of
steel by TiO
2
under UV illumination is highly promising.
This system offers a method of galvanic system without
anode consumption. Photocathodic protection using n-TiO
2
(Nanostructured TiO
2
) film on a steel substrate has shown
to clean the environment while protecting the structural
integrity because of photocatalytic properties of TiO
2
[7].
This paper describes the design of a novel multi
functional cathodic protection system using n-TiO
2
photoanode.
2. THEORY OF PHOTOCATHODIC PROTECTION
The basic idea of photocathodic protection is to replace
the sacrificial anodes such as Mg, Zn or Al with a
semiconductor such TiO
2
and ZnO photoanodes that
generate CB electrons upon band gap irradiation (Fig. 1).
The principle is to use the reductive energy of photo-exited
electrons in the UV irradiated TiO
2
an n-type
semiconductor. On contact with steel, the electrons are
injected to the metal being protected via conduction band.
Hence, the potential of the steel can be polarized in a
direction more negative than the flat band potential of TiO
2
.
If the potential is kept more negative than the corrosion
protection of steel, it can be protected [3, 13]. When TiO
2
was galvanically connected to a steel electrode in the
absence of light the mixed corrosion potential was close to
the Ecorr of steel. However, on illuminating by UV
radiations, the TiO
2
electrode became more negative than
steel because of photo-generated electrons. The counter
reaction is the oxidation of water or any organic
contaminants by photo-generated holes but not the
oxidation of TiO
2
. Hence, TiO
2
photoanode would
continuously discharge current without being consumed
unlike the conventional Zinc or Magnesium anodes. This
makes it an attractive candidate as non-sacrificial anode [5].
Figure 1. Photocatalytic effect- Release of electrons and holes and
production of OH
-
radicals.