Abstract—We compare the photocarrier lifetime measured in
Br-irradiated InGaAs and cold Fe-implanted InGaAsP. We also
demonstrate the possibility of a two-photon absorption (TPA)
process in ErAs:GaAs. The lifetime and the TPA were measured
with a fiber-based 1550 nm time-resolved differential
transmission (ΔT) set-up. The InGaAs-based materials show a
positive ΔT with sub-picosecond lifetime, whereas ErAs:GaAs
shows a negative ΔT consistent with a two-photon absorption
process.
I. INTRODUCTION AND BACKGROUND
HOTOCONDUCTIVE (PC) switches and photomixers are
commonly used for pulsed and CW THz generation. These
devices are based on an ultrafast PC material, which has to
possess a sub-picosecond carrier lifetime to get a short
photocurrent pulse, a high photocarrier mobility to enhance the
emitted THz power, and a high resistivity to allow large bias
voltage in transmitters and reduce the detected noise in
receivers. To achieve such lifetime with standard
semiconductors, defects must be introduced during the growth
or after. Annealed low-temperature-grown (LTG) GaAs is
probably the most widely used THz PC material since it
combines subpicosecond photocarrier lifetime, high resistivity,
and good photocarrier mobility. However, not only is this
material difficult to precisely reproduce, but as a PC switch it
also requires the use of expensive and bulky Ti:sapphire lasers.
GaAs with embedded nanoparticles of erbium (ErAs:GaAs) is
one alternative approach to the LTG GaAs [1], but is usually
driven by lasers near the GaAs band-gap wavelength,
Ȝ 850 nm. There are great advantages to operate THz PC
devices at 1550 nm where lasers are much more affordable
than at 800 nm, and there are catalogues of low-cost fiber-
optic components already well developed for telecom
applications. Nevertheless, the ultrafast PC materials designed
for 1550 nm have generally been inferior to their counterparts
at 800 nm largely because they have been based on
In
0.53
Ga
0.47
As or a similar alloy lattice matched to InP. With
half of the band-gap energy of GaAs, this material generally
suffers from much lower resistivity and breakdown field than
GaAs-based materials. In recent years, however, researchers
have been developing improved 1550-nm materials, such as
Br-irradiated InGaAs [2], ultrafast InGaAs/InAlAs
superlattices [3], and more recently cold Fe-implanted
InGaAsP [4] and 1550-nm-driven ErAs:GaAs [5]. However,
these materials have not been compared in a controlled
fashion. So in this work, we measure and contrast the
1550 nm pump-probe phototransmission signature and
photocarrier relaxation time for three of these materials:
(1) Br-irradiated InGaAs, (2) cold Fe-implanted InGaAsP, and
(3) ErAs:GaAs.
II. SET-UP AND RESULTS
All the measurements were made with the same set-up
shown in figure 1. It consists of a 1550 nm EDFA fiber mode-
locked laser and an optical set-up designed to do time-resolved
differential phototransmission with the same incident power on
each of the samples. The pulse train is delivered by the fiber
laser and split into two parts using a 90/10 fiber splitter. The
pump beam is sent through a U-bench to be chopped at a
frequency around 400 Hz, whereas the probe beam is sent
through a delay line having a maximum relative pump-probe
time delay of 300 ps. After both pump and probe beams pass
through a path-length compensating fiber patch cord, the
beams are focused onto the sample under test using a fiber-to-
free-space coupler. The pulse width at the output of the fiber-
to-free-space coupler (according to optical autocorrelation
measurements) is 250 fs. This is the temporal resolution of the
experiment. The pump power is approximately 140 ȝW, and
the ratio between the pump and probe is about 10.
Fig. 1. Time resolved differential transmission set-up. The pump and the
probe path are the same in time.
Figure 2 shows the differential transmission for the 1-ȝm-
thick Br-irradiated InGaAs sample (on SI-InP substrate) and
the 1.5-ȝm-thick cold-implanted InGaAsP sample (also on SI-
InP substrate) versus the time delay between the pump and the
probe. The data plot of the Br-irradiated InGaAs sample can
be fit by a mono-exponential, yielding τ
1
=400 fs. The cold-
implanted InGaAsP sample is much better fit by two
exponential functions, yielding τ
1
=400 fs and τ
2
=2.2 ps.
Nevertheless, the ratio of the amplitudes of the τ
1
and τ
2
functions is ≈30, which indicates that the τ
2
process
M. Martin
a
, E. R. Brown
a
, J. Mangeney
b
, A. Fekecs
c
, R. Arès
c
, and D. Morris
c
a
Department of Physics, Wright State University, Dayton, OH, 45435, USA
b
IEF, CNRS UMR 8622, Université Paris-Sud, 91405 Orsay Cedex, France
c
Institut Interdisciplinaire d’Innovation Technologique (3iT), Université de Sherbrooke, Sherbrooke, Canada
Email: matthieu.martin@wright.edu
Critical Comparison of Carrier Lifetime at 1.55 ȝm of Ion-Irradiated
InGaAs, Cold-Implanted InGaAsP, and ErAs:GaAs
P
978-1-4673-1597-5/12/$31.00 ©2012 IEEE