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PII:S0960-8524(97)00169-7
Bioresource Technology 64 (1998) 199-204
© 1998 Elsevier Science Ltd. All rights reserved
Printed in Great Britain
0960-8524/98 $19.00
THE APPLICATION OF COLLOIDAL GAS APHRONS IN THE
RECOVERY OF FINE CELLULOSE FIBRES FROM PAPER
MILL WASTEWATER
Mohd. Ali Hashim & Bhaskar Sen Gupta*
Institute of Post Graduate Studies and Research, University of Malaya, 50603 Kuala Lumpur, Malaysia
(Received 23 September 1997; revised version received 27 October 1997; accepted 3 November 1997)
Abstract
Colloidal gas aphrons (CGAs) are micron-sized gas
bubbles of 25-30 kon in diameter produced by a high-
speed stirrer in a vessel containing dilute surfactant
solution. These bubbles, because of their small size,
exhibit some coUoidal properties. In this work, CGAs
were used to separate fine fibres from a lean slurry of
cellulosic pulp in a flotation column. The pulp fibres
were recovered as foamate from the top. Sodium
dodecyl sulphate at a concentration of 2.0 kg/m 3 was
used as a surfactant to generate the CGAs in a
spinning disc apparatus. The results indicated that up
to 70% flotation efficiency could be obtained within a
short column height of 0.3-0.35 m. This technique can
be applied to recover fine cellulosic pulp from paper-
machine backwater © 1998 Elsevier Science Ltd. All
rights reserved
Key words: Flotation, colloidal gas aphrons, cellulose
fibres.
INTRODUCTION
The separation of fine particles, of the order of a
few microns or less, from aqueous media is a
requirement in many chemical and biochemical
processes. Flotation and filtration are the two
common techniques used for this purpose. For
example, a membrane filtration is quite versatile as
it can be employed either to recover the liquid as
permeate or to concentrate the fine particles in the
reject stream. However, it is an expensive process
and is not suitable if recovery of fine particles from
an aqueous medium is the main objective. On the
other hand, flotation is a more economical process
for harvesting fine particles, such as microorganisms
from an aqueous slurry. To this end, the use of
microfoams of colloidal gas aphron dispersions
*Author to whom correspondence should be addressed.
199
(CGAs) is an effective method in recovering fine
particles from a suspension.
Flotation of fine particles by CGAs is recognised
as an inexpensive method of separation. The various
applications of CGAs are as follows (Sebba, 1987;
Subramaniam, 1988):
1. separation of finely divided suspensions of solids
from water
2. removal of finely dispersed oil droplets from
water
3. ion and precipitate flotation
4. removal of ash-forming materials from coal
5. harvesting of microorganisms from a culture
6. clarification of wastewater.
A significant development has taken place in the last
decade on this flotation technique and applications
have been reported in the literature (Subramaniam
et al., 1990; Hashim et al., 1995a,b; Honeycutt et al.,
1983; Save and Pangarkar, 1995).
Colloidal gas aphrons can be described as micron-
sized gas bubbles, of 25-30/~m in diameter, which
are produced by a high-speed stirrer in a vessel
containing dilute surfactant solution. The system was
first termed as 'microfoams' because of the minute
size of the bubbles. These bubbles, because of their
small size and like charges, exhibit some colloidal
properties such as high stability and low coalescence
rates. Hence, microfoams are more commonly desig-
nated as 'colloidal gas aphron dispersions' or CGAs.
The CGAs carry an electrical charge depending on
the surfactant used and combine well with
oppositely charged particles to form a particle-
bubble aggregate, more commonly known as
'foamate', which can be recovered as an overflow.
The entrapped liquid can be separated and recycled
for further CGA generation. The CGAs have the
following properties which are exploited in flotation
processes.
1. Large surface area for particle-bubble contact