Global NEST Journal, Vol 9, No 2, pp 137-143, 2007
Copyright© 2007 Global NEST
Printed in Greece. All rights reserved
TRACING DISPERSED COALY-DERIVED PARTICLES IN MODERN
SEDIMENTS: AN ENVIRONMENTAL APPLICATION OF ORGANIC
PETROGRAPHY
S. KALAITZIDIS
1 1
Department of Geology,
K. CHRISTANIS
1,
* University of Patras, 26500 Rio-Patras, Greece
G. CORNELISSEN
2,3 2
Department of Environmental Engineering,
O. GUSTAFSSON
3
Norwegian Geotechnical Institute (NGI),
P.O. Box 3930 Ullevål Stadion, 0806 Oslo, Norway
3
Department of Applied Environmental Science (ITM),
Stockholm University, 10691 Stockholm, Sweden
*to whom all correspondence should be addressed:
Received: 06/06/06 Fax: +30-2610997560
Accepted: 12/09/06 e-mail: christan@upatras.gr
ABSTRACT
A crucial aspect in environmental sciences is related to the transportation, accumulation and
fate of solid organic particles not native to the sediments. In this study we present the
petrographical features of seven sediment samples obtained from aquatic environments in
Sweden, Finland and The Netherlands. Most of the samples represent the uppermost layers,
which accumulated during the recent past. Their total organic carbon content ranges between
1.5 and 20%. Density separations using heavy liquids were applied, in order to concentrate
the organic matter and thus to facilitate the petrographical determinations. The microscopic
approach revealed significant variations in the origin and hence, the type of the contained
organic matter. Apart from modern plant debris and the algae indicating water-logged
conditions, several particles of naturally and artificially derived solid-organic material were
identified. The latter constitute organic contaminants, and include unburnt residues of high-
rank coals and chars. The petrographic data show a significant comparability with the ‘black
carbon’ data determined by chemo-thermal oxidation at 375°C, demonstrating the applicability
of the microscopic analysis in environmental studies.
KEYWORDS: black carbon, char, fly ash, maceral, environmental organic petrography, solid
coal contamination
INTRODUCTION
A significant field of environmental research concerns the contamination of the natural
environment from industrial activities and particularly from the power generation sector. The
contamination occurs in the form of either solid particles or diluted pollutants (hazardous
and/or toxic organic and inorganic compounds) and originates from mining activities, storage
(e.g. coal/lignite particles), processing and combustion (i.e. combustion derivatives, e.g. fly
ash, unburned residues). The knowledge of the lateral dissemination of these contaminants
and their distribution in the catchments is essential for planning remediation measures.
Moreover, in some areas coaly particles constitute a significant portion of the modern soils
and thus it is necessary to evaluate the fate of these contaminants within the natural eco-
system (e.g. Rumpel et al., 1998, Schmidt et al., 2000, Reyes et al., 2006).
There is a variety of chemical methods to characterize the organic matter in sediments (e.g.
13
C-NMR). However, the heterogeneity of the organic constituents reduces the applicability of
these methods. On the contrary, organic petrography techniques provide the optical
characterization of the organic matter and can aid significantly to the determination of the kind