Delivered by Ingenta to: Korea Advanced Institute of Science & Technology (KAIST) IP : 143.248.247.9 Wed, 13 Oct 2010 12:02:37 Copyright © 2010 American Scientific Publishers All rights reserved Printed in the United States of America Journal of Nanoscience and Nanotechnology Vol. 10, 7212–7216, 2010 Three-Dimensional Spin Configuration of Ferromagnetic Nanocubes H.-G. Piao 12 , D. Djuhana 1 , J.-H. Shim 1 , S.-H. Lee 1 , S.-H. Jun 1 , S. K. Oh 1 , S.-C. Yu 1 , and D.-H. Kim 1 1 BK21 Physics Program and Department of Physics, Chungbuk National University, Cheongju 361-763, South Korea 2 College of Science, Huaihai Institute of Technology, Lianyunguang 222005, China We have systematically investigated three-dimensional spin configurations in ferromagnetic nanocubes using micromagnetic simulation with variation of cube geometry. For thin cuboids, a spin configuration exhibits a four-domain Landau state with a magnetic vortex structure at the center as in the case of a thin film square. For a thick cube, a complex spin configuration with an S-type cylindri- cally asymmetric vortex having two cores on a pair of surfaces while a leaf-like and a C-type states are observed on the other two pairs of cube surfaces. Competition between the geometrical symme- try and magnetic energy minimization condition in ferromagnetic nanocubes leads to the complex spin structure with a spontaneously broken symmetry. Keywords: Ferromagnetic Nanocube, Three Dimensional Spin Configuration. 1. INTRODUCTION Recently, ferromagnetic nanomaterials such as particles, disks, wires, and dots on nanometer scales have attracted great interest for various potential applications in mag- netoelectronics and magnetic recording technology. 1–8 In the patterned ferromagnetic recording media, the ultimate recording density is limited by the superparamagnetic instability originated from the competition between ther- mal fluctuation and ordering magnetization. 9–13 In order to overcome the recording limit, numerous studies have been proposed. For instance, data recording methods using vor- tex core switching or core position in patterned ferromag- netic elements have been proposed, 14–18 while the magnetic vortex structure has been considered to be prevalent in many patterned ferromagnetic system. The magnetic vor- tex in a thin ferromagnetic pattern is composed of a cylin- drically curling spin structure with a vortex core generating the same magnetic surface charges on the patterned film surfaces. 17 On the other hand, very few studies have been addressed to the spin configuration of 3-D nanostructures. One can easily expect that the magnetic vortex structure with core magnetization perpendicular to the patterned film plane will be frustrated, since the core direction is not uniquely determined, for examples, in case of nanocubes due to the unbroken xyz symmetry. Unfortunately, very Author to whom correspondence should be addressed. little has been known for detailed spin configurations in 3-D ferromagnetic nanostructures. In this work, we investigate 3-D spin configuration in fer- romagnetic nanocubes with systematic variation of cuboids thickness by means of micromagnetic simulation, where we observe a transitional behavior of a ground spin configura- tion from a two dimensional simple vortex spin structure to a three dimensional complex spin structure. Full details of 3-D spin configuration in ferromagnetic nanocubes are explored. 2. MICROMAGNETIC SIMULATION Using the object-oriented micromagnetic framework (OOMMF) 19 based on the Landau–Lifshitz–Gilbert equation, 20 3-D spin configurations of various ferromag- netic nanocubes are investigated with systematical variation of cube thickness under the zero external magnetic field. Length and width of the nanocube are set to be 200 nm in all cases. The geometry and dimension of the nanocube are illustrated in Figure 1. The cube thickness d is varied from 5 to 200 nm. In all the micromagnetic simulations, the unit cell dimension is 50 × 50 × 50 nm 3 and the Gilbert damping constant is = 001. The material parameters of Permalloy are chosen to neglect a contribution of magne- tocrystalline anisotropy. The saturation magnetization of M S = 80 × 10 5 A/m and the exchange stiffness coefficient of A = 13 × 10 -11 J/m are used. Initial spin state of a 7212 J. Nanosci. Nanotechnol. 2010, Vol. 10, No. 11 1533-4880/2010/10/7212/005 doi:10.1166/jnn.2010.2760