IOP PUBLISHING JOURNAL OF PHYSICS: CONDENSED MATTER
J. Phys.: Condens. Matter 20 (2008) 184021 (19pp) doi:10.1088/0953-8984/20/18/184021
Bridging the temperature and pressure
gaps: close-packed transition metal
surfaces in an oxygen environment
Catherine Stampfl
1
, Aloysius Soon
1
, Simone Piccinin
1
,
Hongqing Shi
1
and Hong Zhang
1,2
1
School of Physics, The University of Sydney, Sydney New South Wales 2006, Australia
2
School of Physical Sciences and Technology, Sichuan University, Chengdu 610065,
People’s Republic of China
E-mail: stampfl@physics.usyd.edu.au
Received 31 October 2007, in final form 11 February 2008
Published 17 April 2008
Online at stacks.iop.org/JPhysCM/20/184021
Abstract
An understanding of the interaction of atoms and molecules with solid surfaces on the
microscopic level is of crucial importance to many, if not most, modern high-tech materials
applications. Obtaining such accurate, quantitative information has traditionally been the realm
of surface science experiments, carried out under ultra-high vacuum conditions. Over recent
years scientists have realized the importance of obtaining such knowledge also under the high
pressure and temperature conditions under which many industrial processes take place,
e.g. heterogeneous catalysis, since the material under these conditions may be quite different to
that under the conditions of typical surface science experiments. Theoretical studies too have
been aimed at bridging the so-called pressure and temperature gaps, and great strides have been
made in recent years, often in conjunction with experiment. Here we review recent progress in
the understanding of the hexagonal close-packed surfaces of late transition and noble metals in
an oxygen environment, which is of relevance to many heterogeneous catalytic reactions. In
many cases it is found that, on exposure to high oxygen pressures and elevated temperatures,
thin oxide-like structures form which may or may not be stable, and which may have little
similarity to the bulk oxides, and thus possess unique chemical and physical properties.
(Some figures in this article are in colour only in the electronic version)
1. Introduction
The interaction of atoms and molecules with surfaces, and the
chemical processes which occur thereon, play a critical role
in the manufacture and performance of advanced materials
which are used in high-tech applications, for example,
electronic, magnetic, and optical devices, chemical sensors,
heterogeneous catalysts, and hard and corrosion resistant
coatings, to name a but few. In particular, the interaction of
oxygen with transition metals (TMs) is of high importance
for heterogeneous oxidation (and partial oxidation) catalysis
(see e.g. [1–3]) and this has motivated large numbers of early
studies on oxygen–metal interactions [4–6]. Extending atomic
level understanding to elevated temperatures and pressures is
highly desirable, and crucial to understanding the function
of materials that occur under such conditions, but achieving
such knowledge is often not straightforward. For many
heterogeneous catalytic reactions, for example, it is now
established that the characteristics of a material observed
under ultra-high vacuum (UHV) conditions, where classical
surface science techniques dominate, can be expected to be
different to that under the high temperature and pressure
conditions of technical catalysis. In this regime, it is much
more problematic to obtain the same level of microscopic
information. Nevertheless, there remains a general consensus
that the clean metal surface, often assumed to be the catalyst,
may not be the active material phase under such conditions.
Recently, through experimental and theoretical studies
aimed at bridging such gaps, many interesting and significant
findings have been reported; e.g., for the carbon monoxide
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