Effect of Cyclodextrin Derivation and Amorphous State
Complex on Accelerated Degradation of Ziprasidone
JINYANG HONG, JAYMIN C. SHAH, MAURA D. MCGONAGLE
Department of Pharmaceutical Development, Pfizer Global Research and Development, Groton, Connecticut 06340
Received 3 May 2010; revised 21 December 2010; accepted 21 December 2010
Published online 31 January 2011 in Wiley Online Library (wileyonlinelibrary.com). DOI 10.1002/jps.22498
ABSTRACT: Inclusion complexes of ziprasidone with several $-cyclodextrins[$-CDs;
sulfobutylether-$-cyclodextrins (SBE$CD), hydroxypropyl-$-cyclodextrins (HP$CD), methyl-$-
cyclodextrins (M$CD), and carboxyethyl-$-cyclodextrins (CE$CD)] were prepared and solution
stability was evaluated at elevated temperature. Solid-state stability was assessed by subject-
ing various CD complexes of ziprasidone, spray-dried dispersion (SDD), partially crystalline
ziprasidone–SBE$CD salts, and the physical mixture of ziprasidone–SBE$CD to (-irradiation.
Degradant I was formed by oxidation of ziprasidone, which upon aldol condensation with ziprasi-
done formed degradant II in both solution and solid states. In the solution state, CD complexes
with electron-donating side chains, such as SBE$CD and CE$CD, produced the highest oxida-
tive degradation followed by HP$CD with 6, 3, and 4 degrees of substitution. In the solid state,
crystalline drug substance and physical mixture of crystalline drug–SBE$CD showed very lit-
tle to no degradation. In contrast, amorphous $CD, M$CD, CE$CD, and SBE$CD complexes as
well as the amorphous SDD exhibited greatest extent of oxidative degradation. Results suggest
that electron-donating side chains of the derivatized CD interact with transition state of the
oxidation reaction and catalyze drug degradation in solution, However, higher mobility in the
amorphous state of CD–drug complexes promoted chemical instability of ziprasidone under
accelerated conditions irrespective of the chemicalnature of the side chain on CD.© 2011
Wiley-Liss, Inc. and the American Pharmacists Association J Pharm Sci 100:2703–2716,
2011
Keywords: chemicalstability; cyclodextrin;complexation;kinetics; oxidation;solid-state
NMR
INTRODUCTION
Cyclodextrin (CD) has been used in pharmaceuti-
cal formulation as a solubilizer for drug molecules
with low aqueous solubility. CD, with its hydrophobic
cavity and hydrophilic exterior, effectively complexes
with many lipophilic compoundsand thereby in-
creases the aqueous solubility of these compounds.
1–4
Many chemical modifications have been made on CD’s
basic structure to improve its ability to maximize
solubility both in food and drug industry applica-
tions. Many of these modifications involve the intro-
duction of hydrophilic side chains to the exterior of
CD.
3–4
Some noticeable examples of modified CDs are
hydroxypropyl-$-CD (HP$CD) and sulfobutylether-$-
CD (SBE$CD).
3
Correspondence to: Jinyang Hong (Telephone: 860-715-1678;
E-mail: jinyang.hong@pfizer.com)
Journal of Pharmaceutical Sciences, Vol. 100, 2703–2716 (2011)
© 2011 Wiley-Liss, Inc. and the American Pharmacists Association
In addition to solubilization, CD complexation has
been claimed to stabilize drug by protecting the
molecule in the CD cavity and preventing access
of reactive species such as water in hydrolysis of
aspirin.
5
Jarho et al.
6
reported that the deacetyla-
tion of spironolactone in CD complex is pH and CD
dependent, shedding light on the catalytic capability
of derivatized CD on drug degradation. However, the
effects of side-chain electronic and/or steric catalytic
or protective effect on reaction rate of the complexed
drug have not been studied systematically.
Cyclodextrin complexation could affect drug
moleculesin many profound ways. When a drug
molecule is complexed in the CD cavity,the phys-
ical environment is fundamentally different from
either its native crystalline solid state or its simple
solvated state in solution. In addition, complexation
restricts freedom ofthe bound molecule compared
with the bulk drug in solution, and with side chains
in a strategic position on CD that can facilitate the
JOURNAL OF PHARMACEUTICAL SCIENCES, VOL. 100, NO. 7, JULY 2011 2703