Ž . The Science of the Total Environment 213 1998 139150 A historical reconstruction of organic and inorganic contamination events in the Saguenay FjordSt. Lawrence system from preindustrial times to the present Patrick Louchouarn , Marc Lucotte ( ) Chaire de Recherche en Enironnement, HQCRSNGUQAMC.P. 8888, Succ. Centre- ille, Montreal, Que , ´ ´ H3C 3P8, Canada Abstract Based on published chronologies of Hg contamination to the SaguenaySt. Lawrence system as well as sedimen- tary profiles for this heavy metal in the Lower St. Lawrence Estuary, we have established a 100 200 year chronology in the studied sediments and reassessed sedimentation rates for the estuarine system. Our results suggest that sedimentation rates might be higher, by a factor of 1.52, than previously assumed for the Lower Estuary. This chronology in parallel with concentrations of Hg and lignin, the latter an unambiguous marker of terrigenous organic matter, were used successfully to describe natural conditions prevailing prior to the late 19th to early 20th century Ž . and the changes due to industrial activities chlor-alkali, pulp and paper mills that occurred in the first half of the 20th century. In contrast to earlier studies, no significant relationship was found between Hg and lignin in ancient and recent sedimentary intervals contradicting the hypothesis of a particulate lignin-rich carrier-phase controlling the transport and distribution of Hg within the system. Such a correlation between Hg and lignin was only observed in Ž . sediments deposited during a discrete period of high Hg contamination 1940 1975 . However, the covariation of Hg and lignin in sediments deposited in this period results from simultaneous loadings of these two compounds following production growth of chlor-alkali and pulp and paper industries, respectively, and conservative dispersal of sediments from the Upper Saguenay Fjord down to the Lower St. Lawrence Estuary. 1998 Published by Elsevier Science B.V. Keywords: Mercury; Lignin; Saguenay Fjord; Lower St. Lawrence Estuary Corresponding author. 0048-969798$19.00 1998 Published by Elsevier Science B.V. All rights reserved. Ž . PII S0048-9697 98 00085-0