Effect of Nitrate and Sulfate on Dechlorination by a Mixed Hydrogen-Fed Culture 225
1058-8337/02/$.50
© 2002 by CRC Press LLC
Bioremediation Journal 6(3):225–236 (2002)
Effect of Nitrate and Sulfate on Dechlorination by
a Mixed Hydrogen-Fed Culture
D. K. Nelson, R. M. Hozalski, L. W. Clapp, M. J. Semmens, and P. J.
Novak
The Department of Civil Engineering, University of Minnesota, 122 Civil Engineering Building, 500
Pillsbury Drive S.E., Minneapolis, MN 55455–0220
Abstract: A novel hollow-fiber membrane remediation technology developed in our laboratory for hydrogen
delivery to the subsurface was shown to support the dechlorination of perchloroethene (PCE) to cis-dichloroethene.
In previous research, the presence of nitrate or sulfate has been observed to inhibit biological reductive dechlo-
rination. In this study hollow-fiber membranes were used to supply hydrogen to a mixed culture to investigate
whether adequate hydrogen could be added to support dechlorination in the presence of alternative electron
acceptors. By continuously supplying hydrogen through the membrane, the hydrogen concentrations within the
reactor were maintained well above the hydrogen thresholds reported to sustain reductive dechlorination. It was
hypothesized that by preventing nitrate and sulfate reducers from decreasing hydrogen concentrations to below the
dehalorespirer threshold, the inhibition of PCE dechlorination by nitrate and sulfate might be avoided and
dechlorination could be stimulated more effectively. Enough membrane-fed hydrogen was supplied to completely
degrade the alternative electron acceptors present and initiate dechlorination. Nevertheless, nitrate and sulfate
inhibited dechlorinating activity even when hydrogen was not limiting. This suggests that competition for
hydrogen was not responsible for the observed inhibition. Subsequent microcosm experiments demonstrated that
the denitrification intermediate nitrous oxide was inhibitory at 13 μM.
Key Words: dechlorination, hollow-fiber membranes, hydrogen, nitrate, sulfate, electron donor.
Introduction
The contamination of aquifers with chlorinated solvents
such as perchloroethene (PCE) has emerged as a major
problem over the last few decades. One technique for
remediating these contaminated aquifers is in situ anaero-
bic biological reductive dehalogenation. Indigenous mi-
croorganisms are capable of mediating the reduction of
chlorinated solvents such as PCE via either a gratuitous
process or via a process termed dehalorespiration, where
microorganisms are able to conserve the energy pro-
duced during PCE reduction (Holliger, 1993; Neumann
et al., 1994). The reduction of chlorinated solvents is
often limited in situ by a lack of electron donor. Based
on this concept, several technologies have been used to
supply excess electron donor to contaminated sites to
stimulate biological reductive dehalogenation. These
include the addition of fermentable substrates (Carr and
Hughes, 1998; Fennell et al., 1997; Fennell and Gossett,
1998) and direct sparging of hydrogen gas (H
2
) (Hughes
et al., 1997).
One novel technology that has been developed
recently is the use of gas-permeable hollow-fiber mem-
brane modules to continuously supply H
2
directly to
groundwater (Fang et al., 2002; Muenzner et al., ac-
cepted). Membrane modules can be designed to pro-
vide a large surface area for passive gas transfer while
presenting minimal resistance to hydraulic flow. This
innovative gas transfer technology overcomes the prob-
lems of conventional gas transfer devices: inefficiency,
nonuniform delivery, and gas loss, by dissolving H
2
directly into the water without bubble formation (Côté
et al., 1988; Côté et al., 1989; Ahmed and Semmens,
1992a). These membranes are capable of achieving
100% gas transfer efficiency (Ahmed and Semmens,
1992a; Ahmed and Semmens, 1992b). In addition, the
resulting dissolved H
2
concentration in the water can
be controlled precisely by adjusting membrane surface
area and gas pressure (Semmens and Gantzer, 1993).
Thus, gas-permeable membranes appear to be a suit-
able method for providing H
2
as an electron donor for
in situ biological dehalogenation.