Activation and Stabilization of Penicillin V Acylase from
Streptomyces lavendulae in the Presence of Glycerol and Glycols
Miguel Arroyo,* Raquel Torres-Guzma ´ n, Isabel de la Mata, M. Pilar Castillo ´ n, and
Carmen Acebal
Departamento de Bioquı ´mica y Biologı ´a Molecular I, Facultad de Ciencias Biolo ´gicas,
Universidad Complutense de Madrid, Spain
Penicillin V acylase (EC 3.5.1.11) from Streptomyces lavendulae showed both enhanced
activity and stability in mixed water/glycerol and water/glycols solvents. The catalytic
activity was increased up to a critical concentration of these cosolvents, but further
addition of the latter led to a gradual protein deactivation. The highest stabilizing
effect was achieved in the presence of glycerol. Thermal stability was increased
proportionally to the concentration of glycerol and glycols in the reaction mixture only
if the amount added is below the threshold concentration. Reaction conditions that
allow simultaneously enhanced activity and stability in the hydrolysis of penicillin V
catalyzed by penicillin V acylase from S. lavendulae could be established.
Introduction
Nonaqueous enzymology has greatly expanded the
potential scope and economic impact of biocatalysis,
opening a new field in the biotechnological applications
of enzymes (Gupta, 1992). Enzymatic activity sometimes
may be improved as a result of the incorporation of a
small amount of a water-miscible organic solvent in the
reaction mixture (Tan and Lovrien, 1972; Batra and
Gupta, 1994). However, aqueous-organic monophasic
systems have not become very popular because many
water-miscible organic solvents can act as denaturing
agents for proteins at moderate concentrations (Mozhaev
et al., 1989). Despite this, there are some polyhydric
cosolvents that may improve enzyme stability. These
cosolvents such as glycerol and glycols, are well-known
protective agents against thermal denaturation, and they
are less deleterious at high concentrations in the reaction
medium (Mozhaev et al., 1989). In particular, glycerol is
known to be a strong stabilizing agent of biomolecules
(Gekko and Timasheff, 1981a) and is widely employed
for storing proteins and enzymes. In 1991, Khmelnitsky
and co-workers introduced a new parameter called
denaturation capacity (DC), which indicates the protein
denaturing strength of an organic solvent on a scale from
0 to 100. In the DC scale of Khmelnitsky, glycerol and
ethylene glycol have very low DC values (20.2 and 18.7,
respectively), meaning that these solvents exert the least
denaturing effect on proteins. In this work, we have
systematically studied the effect of increasing the con-
centrations of glycerol, ethylene glycol, diethylene glycol,
and triethylene glycol on the activity and stability of
penicillin V acylase (PVA) from Streptomyces lavendulae.
This enzyme catalyzes the hydrolysis of penicillin V to
yield 6-amino penicillanic acid (6-APA), an important key
intermediate of semisynthetic penicillins (Shewale and
Sudakaran, 1997). The use of water/glycerol and water/
glycol mixtures can enhance the hydrolysis rate of
penicillin V catalyzed by PVA, in addition to improving
its thermal stability. The present work describes a useful
medium in the manufacture of 6-APA employing PVA
from S. lavendulae.
Experimental Section
Enzyme Production and Partial Purification.
Penicillin V acylase (EC 3.5.1.11) was produced from S.
lavendulae (ATCC 13664) by fermentation (Torres et al.,
1999), and it was purified 30-fold with a yield of 26.4%
as reported elsewhere (Torres et al., 1998).
Enzyme Activity. The potassium salt of phenoxy
methyl penicillin (PVK) from Sigma (St. Louis, MO) was
used as substrate in the enzyme assays. A 50 µL sample
of the purified PVA solution was mixed with 85 µL of
water, 15 µL of 1 M potassium phosphate buffer (pH )
8.0), and 150 µL of a PVK solution (45 mg/mL) in water.
The reaction mixture was incubated for 30 min at 40 °C
under gentle shaking. The reaction was stopped by
addition of 0.9 mL of 20% (v/v) acetic acid solution. The
reaction mixture was centrifuged, and a 0.9 mL aliquot
was processed for estimation of 6-APA by addition of 300
µL of a 0.5% (p/v) solution of p-dimethylamino benzal-
dehyde (Sigma Chemical Co., St. Louis, MO) in methanol
(Shewale et al., 1987). One activity unit is defined as the
amount of enzyme producing 1 µmol/min of 6-APA under
the assay conditions. Previous kinetic analyses were
performed to make sure that the activity was linear in
the assay conditions for 30 min (in buffer and in the
presence of cosolvents) using the saturating concentration
of penicillin V described above. We employed an enzyme
solution with an activity of 1.0 unit/mg protein in all the
assays.
Effect of Glycerol and Glycols on Enzyme Activ-
ity. The effect of glycerol, ethylene glycol, diethylene
glycol, and triethylene glycol (Merck, Germany) on
penicillin V acylase activity at different solvent concen-
trations was analyzed. The solvents were incorporated
into 50 µL of enzyme solution prior to the addition of
penicillin V. The volume of water was corrected for the
added solvent so that the volume remained 150 µL. The
enzyme activity, in contact with the solvent, was mea-
sured after the addition of 150 µL of PVK solution, so * Tel: (+34) 91-394 41 50. Fax: (+34) 91-394 46 72.
368 Biotechnol. Prog. 2000, 16, 368-371
10.1021/bp000023h CCC: $19.00 © 2000 American Chemical Society and American Institute of Chemical Engineers
Published on Web 05/16/2000