Ian David Lockhart Bogle and Michael Fairweather (Editors), Proceedings of the 22nd European
Symposium on Computer Aided Process Engineering, 17 - 20 June 2012, London.
© 2012 Elsevier B.V. All rights reserved
Multiobjective Optimization in Distillation with
Reactor-Side for Hydrodesulfurization Process of
Diesel
Erick Y. Miranda-Galindo
a
, Juan G. Segovia-Hernández
a
, Salvador Hernández-
Castro
a
, Adrián Bonilla-Petriciolet
b
and Gade Pandu Rangaiah
c
a
Universidad de Guanajuato, Campus Guanajuato, Division de Ciencias Naturales y
Exactas, Departamento de Ingenieria Quimica, Noria Alta S/N, Guanajuato, Gto.,
36050, Mexico
b
Instituto Tecnológico de Aguascalientes, Departamento de Ingeniería Química,
Aguascalientes, 20256, México
c
National University of Singapore, Department of Chemical & Biomolecular
Engineering, Engineering Drive 4, 117576, Singapore
Abstract
The distillation reactor-side has been proposed to remove sulfur compounds of diesel.
The design and optimization of a hydrodesulfurization process involve the selection of
the configuration and the operating conditions to minimize the total annual cost, CO
2
emissions and the amount of sulfur compounds. In general, the optimal design of
hydrodesulfurization process is a highly non-linear and multivariable multiobjective
optimization problem, with the presence of both continuous and discontinuous design
variables. In particular, stochastic multiobjective optimization algorithms are capable of
solving, robustly and efficiently, challenging optimization problems, and they appear to
be a suitable alternative for the design and optimization of complex process schemes. In
this study, we have implemented a multi-objective optimization method to obtain the
design and optimization of three distillation reactor-side in the hydrodesulfurization
process. The results obtained in the Pareto Fronts indicate competition between total
annual cost, CO
2
emissions and the amount of sulfur compounds of the
hydrodesulfurization process. These Pareto Fronts are useful to identify proper
conditions for the operation of this process. In general, the reduction of the amount of
sulfur compounds increases the TAC and CO
2
emissions. However, we can identify
operating conditions where the TAC can be reduced.
Keywords: hydrodesulfurization process, multiobjective optimization, Pareto Front.
1. Introduction
The design of new processes in the chemical engineering industry takes into account
policies of process intensification, which can be defined as any chemical engineering
development that leads to a substantially smaller, cleaner, and more energy-efficient
technology. One example of process intensification is the minimization of total annual
cost (TAC), which is associated with lower energy consumption, lower greenhouse gas
emissions, miniaturization of process equipment, multipurpose equipment, safety
operations, and others (Moulijn et al., 2008). In particular, hydrodesulfurization (HDS)