Appl. Phys. A 58, 541-549 (1994)
Applied ,o,,,,,
Physics A-" Surfaces
© Springer-Verlag 1994
On the Influence of Extrinsic Point Defects on Irradiation-Induced
Point-Defect Distributions in Silicon
J. Vanhellemont, A. Romano-Rodriguez*
IMEC, Kapeldreef 75, B-3001 Leuven, Belgium (Fax: +32-16/281501)
Received 18 November 1993/Accepted22 February 1994
Abstract. A semi-quantitave model describing the in-
fluence of interfaces and stress fields on {ll3}-defect
generation in silicon during 1-MeV electron irradiation,
is further developed to take into account also the role of
extrinsic point defects. It is shown that the observed
distribution of { 113}-defects in high-flux electron-irradi-
ated silicon and its dependence on irradiation tempera-
ture and dopant concentration can be understood by tak-
ing into account not only the influence of the surfaces
and interfaces as sinks for intrinsic point defects but also
the thermal stability of the bulk sinks for intrinsic point
defects. In heavily doped silicon the bulk sinks are related
with pairing reactions of the dopant atoms with the
generated intrinsic point defects or related with enhanced
recombination of vacancies and self-interstitials at ex-
trinsic point defects. The obtained theoretical results are
correlated with published experimental data on boron-
and phosphorus-doped silicon and are illustrated with
observations obtained by irradiating cross-section trans-
mission electron microscopy samples of wafers with
highly doped surface layers.
PACS: 61.80.Fe, 61.70.Bv, 61.70.Yq
Irradiation of electronic devices with high energy parti-
cles leads to a degradation of the device characteristics
which is partly due to the creation of lattice damage in
the active areas of the devices. A convenient way of
studying the basic mechanisms of the formation of radia-
tion-induced displacement damage is irradiation with
MeV electrons which is known to create individual in-
trinsic point defects rather than extensive collision cas-
cades. Low flux electron irradiation leads to the forma-
tion of point defect complexes such as divacancies and
dopant/intrinsic point defect pairs. High fluxes of MeV
* Permanent address: LCMM, Departament de Fisica Aplicada i
Electrbnica, Universitat de Barcelona, Diagonal 647, E-08028 Bar-
celona, Spain
electrons create a supersaturation of self-interstitials
which cluster in so-called {ll3}-defects which can be
observed in situ during irradiation in a High-Voltage
transmission Electron Microscope (HVEM). The distri-
bution of {113}-defects in the irradiated sample can be
used to monitor local variations of the intrinsic point-
defect concentration.
Already in 1981, Brown and Fathy [1] observed a
strong dependence of { 113}-defect generation on the type
and the concentration of dopant atoms. Aseev and co-
workers [2-5] have studied this phenomenon in more
detail using silicon samples doped with different con-
centrations of boron or phosphorus atoms. Recently,
experimental results were also obtained by the present
authors by irradiating cross-section samples of wafers
with a dopant concentration depth profile [6-9]. The
impact of interfaces and localised mechanical stress fields
on the {ll3}-defect distribution was discussed in a
previous paper in which a first order model was presented
to explain the generation of {ll3}-defects near TEM
specimen surfaces and interfaces [10].
Other extrinsic point defects which are not electrically
active play also an important role in the {ll3}-defect
nucleation and growth. Hua et al. [11, 12] showed that
interstitial oxygen enhances the { 113}-defect nucleation,
which is much lower in oxygen lean FZ material. The
experiments of Hasebe et al. [13] and by the present
authors [7] demonstrated the important impact of carbon
diffusing in from the specimen surface and leading to an
enhanced initial defect formation near this surface. Ni-
trogen on the contrary is reported to suppress strongly
{ll3}-defect nucleation even for a nitrogen concentra-
tion as low as 1015 cm -3 [14]. A similar suppression of
defect formation is observed in germanium-doped silicon
or in silicon/germanium alloys [8, 15].
In the present study an attempt is made to extend the
first order model of [10] to explain also the observations
obtained after irradiation in a high voltage transmission
electron microscope of plan view and cross-section spe-
cimens of highly doped silicon. It is shown that the
published data on {113}-defect generation in uniformly