FULL PAPER
DOI: 10.1002/ejic.200801068
Transformation of Solid Potassium Ferrate(VI) (K
2
FeO
4
): Mechanism and
Kinetic Effect of Air Humidity
Libor Machala,
[a]
Radek Zboril,*
[a]
Virender K. Sharma,
[b]
Jan Filip,
[a]
Dalibor Jancik,
[a]
and Zoltan Homonnay
[c]
Keywords: Solid-state reactions / Iron / Reaction mechanisms / Environmental chemistry / Moessbauer spectroscopy
The kinetics of solid-state transformation (aging) of potas-
sium ferrate(VI) (K
2
FeO
4
) under various air-humidity condi-
tions (55–95 % relative humidity) at room temperature were
studied by in-situ Mössbauer spectroscopy. The kinetic data
showed a significant increase in the decomposition rate with
increasing air humidity. The decomposition kinetics is very
unusual with two almost linear decay steps. The first slow
decay was observable at rather lower humidity levels (55–
70 %) probably due to the formation of the narrow compact
layer of nanoparticulate Fe(OH)
3
reaction product. This layer
limits the access of both H
2
O and CO
2
participating in the
reaction as the gaseous reactants. The second decay with
much faster rate showed a nearly positive linear relationship
with the humidity. The identification and characterization of
the final products of aging were conducted by using X-ray
Introduction
Iron(VI) compounds [ferrates(VI), FeO
4
2–
] represent an
advanced class of compounds, which can be used in many
promising electrochemical, environmental, and chemical
applications such as high-energy-density rechargeable bat-
teries
[1–5]
and cleaner (“greener”) technologies of organic
syntheses,
[6–8]
“environmentally friendly” oxidant useful in
innovative technologies for water treatment.
[9–24]
Among
multitudes of other advantageous properties it is worth to
emphasize the coagulation and disinfection ef-
fects.
[11,12,25–28]
The wide range of applications induced a great effort to
prepare ferrate(VI) of sufficient purity on a large scale. Up
to now, several synthetic routes were developed including
[a] Centre for Nanomaterial Research and Departments of Experi-
mental Physics and Physical Chemistry, Palacky University in
Olomouc,
Svobody 26, 77146 Olomouc, Czech Republic
Fax: +420-58-563-4958
E-mail: zboril@prfnw.upol.cz
[b] Chemistry Department, Florida Institute of Technology,
150 West University Boulevard, Melbourne, Florida 32901,
USA
[c] Department of Nuclear Chemistry, Eötvös Loránd University,
Pázmány P. s. 1/A, 1117 Budapest, Hungary
Supporting information for this article is available on the
WWW under http://www.eurjic.org or from the author.
© 2009 Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim Eur. J. Inorg. Chem. 2009, 1060–1067 1060
diffraction (XRD), variable-temperature and in-field Möss-
bauer spectroscopy, magnetic measurements, thermogravim-
etry (TG) and differential scanning calorimetry (DSC), and
scanning electron microscopy (SEM) techniques. The reac-
tion mechanism, assuming formation of KHCO
3
and Fe(OH)
3
in the molar ratio of 2:1 per 1 mol of solid K
2
FeO
4
was sug-
gested. The SEM images revealed the formation of large
KHCO
3
crystallites whose surface was covered by ultrasmall
X-ray amorphous iron(III) hydroxide nanoparticles in a high
degree of agglomeration. The obtained results of aging un-
der humid conditions are important for the possible storage
of K
2
FeO
4
and thus for its environmental and industrial ap-
plications.
(© Wiley-VCH Verlag GmbH & Co. KGaA, 69451 Weinheim,
Germany, 2009)
chemical, electrochemical, and thermal techniques.
[29–35]
Regardless of the synthetic route, ferrate(VI) salts are rela-
tively stable over a long period of time if stored in a dry
atmosphere. However, they become quite unstable if treated
at high temperatures
[36]
and/or if exposed to air humidity
even at room temperature.
[37]
The decomposition mechanism and stability of hexa-
valent iron compounds have been investigated in solu-
tions,
[4,38–42]
whereas the solid-state room-temperature
transformation has been reported only by Nowik et al.
[37]
The authors studied the disintegrations of solid K
2
FeO
4
and BaFeO
4
samples sealed and exposed to dry and/or hu-
mid air. Mössbauer spectroscopy was applied to identify
the possible intermediate oxidation states (V, IV) of iron
and to characterize the final iron-bearing products.
[37]
In
the case of K
2
FeO
4
, the final formation of Fe
2
O
3
nanopar-
ticles was suggested in both atmospheres, and no intermedi-
ates containing iron in higher valence states were detected.
The potassium-containing reaction product has not been
determined at all.
[37]
The detailed analytical approach used in this paper pro-
vides evidence of the formation of KHCO
3
and amorphous
Fe(OH)
3
as the aging products (molar ratio of 2:1) of
K
2
FeO
4
in humid air. This newly suggested reaction mecha-
nism, assuming participation of the H
2
O and CO
2
gaseous
reactants, fills a gap in basic inorganic chemistry of high