Cellular Behaviors on Chemically/Physically
Modified SiO
2
Surfaces
Chung-Yao Yang
1
, Amarendra Kumar
1
, J. Andrew Yeh
1
Insitute of Engineering and Microsystems
National Tsing Hua University
Hsinchu, Taiwan
d9535803@oz.nthu.edu.tw
Yao-Joe Yang
Department of Mechanical Engineering
National Taiwan University
Taipei, Taiwan
Abstract—This paper describe an easy-to-handle approach to
probe cellular behaviors via using silicon dioxide nanotextures
with various functional groups. The silicon dioxide nanotextures
were performed through using metal assisted chemical etching
and wet oxidation. The pitch of nanotextures can be adjusted by
controlling etching durations. The results showed that cells
preferred to spread out on nanotextures with longer pitch rather
than on nanotextures with shorter pitch. In addition, cells also
preferred to adhere on planar surface rather than on
nanotextured surface. We believe, this study can help us to get
more insights of cell biology and biomedical-relevant researches.
Keywords—nanostructures; glass; functional group; cellular
behavior; cell morphology
I. INTRODUCTION
Cell behaviors such as growth, differentiation, migration and
death can be influenced by the cell interaction with the
surrounding environments. There are various
pathways/mechanisms that regulate how a cell senses and
replies to the surrounding environments. These include cell-
based properties (e.g., integrin-ligand interactions), physical
cues (e.g., topographical influences of the surface) and
chemical cues (e.g., effects of surface chemistry). The ability
to understand and, further, control or modulate cell-substrate
interactions (or cell-material interfaces) through
transmembrane receptors such as integrin has provided us a
more comprehensive understanding of cellular responses
associated with the physiologically/pathologically relevant
microenvironment wherein single cells attach and spread,
coherently linking to cell structural properties and responses.
Furthermore, maintaining deregulation and homeostasis which
can lead to disease are important under these
microenvironmental conditions [1].
There is still a challenge to be solved which is the
signaling pathway of focal adhesion based on single protein
assembly in the research field of cell adhesion. In particular,
the mechanism of cell adhesion and the size/shape of focal
adhesion cluster are still mysteries in cell biology. Using
micro-/nano-technology combined tools to manipulate these
processes in focal adhesion would allow us to regulate cell
adhesion in the future. Nano-textured substrates have been
shown to significantly influence migration [2], cell adhesion
and gene expression [3,4]. The ability of cells to respond to a
variety of factors dictates ultimate cell behaviors including
proliferation and apoptosis. Numerous researches show that
cell-cell interaction in cancer cell lines may be correlated with
the regulation of angiogenesis [5,6]. It is crucial to explain
how the molecular pathways of angiogenesis resulting in
cancer disease, and this knowledge can be used to design
suitable drugs for more efficient therapies. Nano-fabricated
surfaces with several nanometer scale textures have potentially
provided physical-based biocompatible tools to manipulate the
arrangement of various cells for studying cell-cell interaction.
For investigating cell-substrate/cell-cell interactions of human
cancer cells on nanometer scale textures, we provided an easy-
to-handle and chemical-based etching to imitate the in vivo
environment and functionalize the surfaces with different
functional group chemicals with respect to cell-substrate
interaction.
The most common surface modification scheme for
materials is reaction of alkylchlorosilanes with water and/or
surface hydroxyl groups in a solution-based process to form a
thin alkylsilane film. This process highly depends on reaction
temperature, silanol species in solution, and nature of the
solvent. Additionally, liquidbased coating process is a time-
consuming process and may influence the topography of nano-
scale features due to the unsolved molecules in solution.
Vapor-phase coating processes via volatile fluorinated
alkylsilanes has been demonstrated [7,8], which offers several
advantages, compared to liquid-based approaches, which
inherently have several major issues including (i) diffusion
limited transport of reagents into specific areas, (ii) incomplete
wetting of high-aspect ratio structures, (iii) control of dissolved
water in non-aqueous solvents, (iv) uncertain reaction in
solution, and (v) disposal of solvent waste. Vapor-phase
process provides distinct advantages such as (i) efficient
transport into high-aspect ratio structures, (ii) no solvent waste,
(iii) good control of reagent, and (iv) provide convenient, in
situ cleaning prior to deposition. According to these reasons,
cell behavior on nanostructures with/without chemicals is
unclear due to the liquid phase chemicals may change the
topography of nanostructures.
Recently, numerous studies have been carried out to
fabricate nanostructures on quartz wafer through dry etching
approach (i.e., reactive ion etching, inductively coupled plasma,
978-1-4799-4726-3/14/$31.00 © 2014 IEEE
655
Proceedings of the 9th IEEE International
Conference on Nano/Micro Engineered and Molecular Systems
April 13-16, 2014, Hawaii, USA