ISSN 0003-701X, Applied Solar Energy, 2014, Vol. 50, No. 4, pp. 255–259. © Allerton Press, Inc., 2014.
Original Russian Text © B.L. Oksengendler, O.B. Ismailova, M.B. Marasulov, I.Z. Urolov, 2014, published in Geliotekhnika, 2014, No. 4, pp. 55–59.
255
INTRODUCTION
Among various problems of photovoltaics, most
recently the special interest of researchers has been
attracted to solar cells based on perovskites based on
organic–inorganic components; in the most general
terms this is CH
3
NH
3
PbJ
3
or close variants [1]. The
start of the “perovskite era” (see [2]) occurred in 2009
[3]; then, over 2012–2013 the conversion rate of solar
energy into electrical energy increased from 10% [4] to
15% [5]. To date, the characteristic physical and
mechanical structure of a perovskite solar cell
(Figs. 1a, 1b, 1c, 1d) has been formed, which is char-
acterized by the corresponding electronic band struc-
ture of the device (Fig. 1b). Along with excellent fea-
tures of perovskite cells (inexpensive and relatively
simple low-temperature technology and an under-
standable physical chemistry of the components),
some difficulties have been identified, whose solution
could lead, according to some experts [2], to a “new
On the Degradation Mechanism of Functioning Solar Cells
Based on Organic–Inorganic Perovskites
B. L. Oksengendler
a
, O. B. Ismailova
b
, M. B. Marasulov
a
, and I. Z. Urolov
a
a
Institute of Polymer Chemistry and Physics, Academy of Sciences of the Republic of Uzbekistan, Uzbekistan
b
Institute of Ion-Plasma and Laser Technologies, Academy of Sciences of the Republic of Uzbekistan, Uzbekistan
e-mail: oksengendlerbl@yandex.ru
Received March 23, 2014
Abstract—This paper presents the first attempt to build a model and detect the degradation mechanism of
organic–inorganic photovoltaic solar cells based on perovskites. The cross section of the process of the for-
mation of a close Frenkel pair in the sublattice of iodine is obtained and its annealing channels are found. It
is concluded that there is a nonmonotonic dependence of the stationary number of defects on the intensity
of solar radiation, which allows one to analyze the properties of the radiation resistance of a device to ionizing
radiation.
DOI: 10.3103/S0003701X14040100
HELIOTECHNICAL
MATERIALS SCIENCE
(100 nm)
Energy
vacuum
(c) (d)
Au
PCBM
CH
3
NH
3
PbJ
3
PolyTPD
PEDOT:PSS
ITO
(a)
(b)
(10 nm)
(285 nm)
(10 nm)
(70 nm)
ITO
PEDOT:PSS
–4.8
–2.4
–3.9
–5.4
–5.9
–5.4 –5.4
–5.3
–3.9
Au
PC BM CH
3
NH
3
PbJ
3
PolyTPD
OCH
3
O
N N
n
Fig. 1. The scheme of a solar cell based on perovskite: (a) the geometric structure of layers; (b) the electronic structure of layers;
(c) the chemical structure of polerelomin (polyTPD); (d) the chemical structure of PCBM (see [1–3]).