Hardness of Nanocrystalline TiO
2
Thin Films
Danuta Kaczmarek
1,a
, Jaroslaw Domaradzki
1,a
, Damian Wojcieszak
1,a
,
Eugeniusz Prociow
1,a
, Michal Mazur
1,a
, Frank Placido
2,a
, Steffen Lapp
2,a
1
Faculty of Microsystem Electronics and Photonics, Wroclaw University of Technology,
Janiszewskiego 11/17, 50-372 Wroclaw, Poland
2
University of the West of Scotland, High Street, Paisley, PA1 2BE,
and SUPA, Scottish Universities Physics Alliance, United Kingdom
a
damian.wojcieszak@pwr.wroc.pl (corresponding author)
Keywords: hardness, nanocrystalline, TiO
2
, thin film, nanoindentation
Abstract. In this work results of hardness investigations of nanocrystalline TiO
2
thin films are
presented. Thin films were prepared by low pressure hot target reactive sputtering (LPHTRS) and
high energy reactive magnetron sputtering (HERMS). In both processes a metallic Ti target was
sputtered under low pressure of oxygen working gas. After deposition by LPHTRS TiO
2
thin films
with anatase structure were obtained and after additional post-process annealing at 1070 K, these
films recrystallized into the rutile structure. Annealing also resulted in an increase of average
crystallite size from 33 nm (for anatase) to 74 nm (for rutile). The HERMS process is a
modification of the LPHTRS process with the addition of an increased amplitude of unipolar
voltage pulses, powering the magnetron. This effectively increases the total energy of the depositing
particles at the substrate and allows dense, nanocrystalline (8.7 nm crystallites in size) TiO
2
thin
film with the rutile structure to be formed directly.
The hardness of the films was determined by nanoindentation. The results showed that the
nanocrystalline TiO
2
-rutile thin film as-deposited using HERMS had high hardness (14.3 GPa),
while the TiO
2
-anatase films as-deposited by LPHTRS, were 4-times lower (3.5 GPa). For
LPHTRS films recrystallized by additional annealing, the change in thin film structure from anatase
to rutile resulted in an increase of film hardness from 3.5 GPa to only 7.9 GPa. The HERMS
process can therefore produce the TiO
2
rutile structure directly, with hardness that is 2 times greater
than rutile films produced by LPHTRS with additional annealing step.
Introduction
Nowadays, for many commercial products high resistance against external hazards is often required.
Especially, hardness is one of the most important parameters, resulting in many devices being
coated with different so called hard coatings. Recent research has shown that coatings with
nanocrystalline structures have greatly increased hardness compared to the non-crystalline coatings
that are usually applied in the coating industry [1]. Such coatings, besides their protective function,
are often required to satisfy many other requirements, for example: excellent transparency in the
visible range [2], high photocatalytic activity [3], wettability (hydrophobic or hydrophilic
properties) [4, 5]. For these reasons, well known optical coatings such as SnO
2
[6], ZrO
2
[7], SiO
2
[8] and TiO
2
[9] are good candidates for hard coatings. Apart from the intrinsic material differences,
in practise the application of different process parameters [10], additional post-process treatment
(e.g. annealing) [11] or doping with different elements [12] also allow the properties of thin film
coatings to be varied. Of these, modification of the film structure during thin film deposition seems
to be the most desirable and important route since it allows significantly new structural properties
that can not readily be achieved by post-deposition treatments.
In this work the influence of deposition process parameters on the hardness of nanocrystalline
TiO
2
thin films have been investigated. Thin films were manufactured by two so called hot-target
reactive magnetron sputtering processes. The main difference between the two was the amplitude of
the magnetron power supply [13, 14]. While films prepared by the low pressure hot target reactive
Journal of Nano Research Vols. 18-19 (2012) pp 195-200
Online available since 2012/Jul/26 at www.scientific.net
© (2012) Trans Tech Publications, Switzerland
doi:10.4028/www.scientific.net/JNanoR.18-19.195
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