TETRAHEDRON
LETTERS
Tetrahedron Letters 42 (2001) 3243–3246 Pergamon
Effect of temperature on peptide chain aggregation: an EPR
study of model peptidyl-resins
Suely C. F. Ribeiro,
a
Shirley Schreier,
b
Clovis R. Nakaie
a
and Eduardo M. Cilli
a,
*
a
Department of Biophysics, Universidade Federal de Sa ˜o Paulo, Rua 3 de Maio 100, 04044 -020, Sa ˜o Paulo, SP, Brazil
b
Department of Biochemistry, Institute of Chemistry, Universidade of Sa ˜o Paulo, C.P. 26077, 05513 -970, Sa ˜o Paulo, SP, Brazil
Received 9 February 2001; revised 6 March 2001; accepted 12 March 2001
Abstract—The effect of temperature on the dynamics of peptide chains inside resin beads was monitored by electron paramagnetic
resonance (EPR) spectroscopy. A two-component spectra was obtained for low and highly peptide-loaded model peptidyl-resins
labeled with the paramagnetic aminoacid 2,2,6,6-tetramethyl-piperidine-N-oxyl-4-amino-4-carboxylic acid (TOAC), indicating the
presence of strongly and weakly immobilized populations. Increasing levels of chain disaggregation were observed with increasing
temperature, leading in some cases to a complete disappearance of the more immobilized population. The present findings
demonstrate that EPR spectral parameters are highly sensitive to the solvation properties of labeled sites inside the resin matrix
and can be of great value for the understanding of polymer-supported processes or reactions. © 2001 Elsevier Science Ltd. All
rights reserved.
Merrifield’s solid-phase peptide synthesis method
1
has
been intensively investigated as a convenient model to
improve the knowledge of the physicochemical basis of
processes occurring throughout a polymeric matrix. In
this context, emphasis has been recently given to resin-
supported combinatorial chemistry for the development
of new drugs.
2,3
Despite all these continuous efforts to
optimize the peptide synthesis protocol, serious short-
comings have intriguingly persisted. They are mainly
related to incomplete coupling during peptide growth
caused by chain aggregation inside the bead.
4
To over-
come this problem alternative solid supports have been
continuously proposed for peptide synthesis.
5,6
In addi-
tion, attempts to establish the rules which govern resin
solvation have been the object of several publications,
as this property has been found to depend upon the
Figure 1. Effect of temperature upon the EPR spectra of TOAC-labeled low (A) and highly loaded (B) VQAAIDYING-BHAR
in DMF.
* Corresponding author. E-mail: cilli.biof@infar.epm.br
0040-4039/01/$ - see front matter © 2001 Elsevier Science Ltd. All rights reserved.
PII:S0040-4039(01)00414-2