Thin Solid Films, 164 (1988) 217 220
217
AN INTERESTING UNCONVENTIONAL PHOTOINDUCED CHANGE
IN THE DARK CONDUCTIVITY OF a-Si:F:H*
S. C. DE, GAUTAM GANGULY, SWATI RAY AND A. K. BARUA
Energy Research Unit, Indian Association for the Cultivation of Science, Jadavpur, Calcutta 700032
(India)
The results of light exposure on dark conductivity, its activation energy, and the
photoconductivity of a-Si:F:H samples are presented. A light-induced decrease in
photoconductivity by a factor of about 3 is observed. The changes in dark
conductivity are rather unusual. The direction of the change is found to depend on
the position of the Fermi level. At a particular activation energy (about 0.85 eV) no
light-induced change in the dark conductivity occurs. This behaviour has been
explained in terms of a model. The temperature dependence of the defect creation
and annealing has also been reported.
1. INTRODUCTION
Light-induced changes in the opto-electronic properties 1 and the consequent
degradation of the performance of amorphous silicon thin-film photovoltaic
devices 2 has been an active area of research. One of the reasons for the interest in
fluorinated hydrogenated amorphous silicon thin films, first prepared by Ovshinsky
and Madan 3, has been the reduced light-induced metastable changes in the
properties of the material 4. Extensive study of the properties of a-Si:F:H as a
function of the deposition parameters 4' 5 has established that device quality material
can be prepared by the glow discharge deposition technique. We have undertaken
an intensive study of the effects of light soaking on the dark conductivity, activation
energy and photoconductivity of a-Si:F:H thin films. Here, we report mainly the
unusual changes in the dark conductivity and activation energy observed in
a-Si:F:H films deposited by the r.f. glow discharge deposition technique.
2. EXPERIMENTAL DETAILS
The a-Si:F:H samples were prepared from mixtures of silicon tetrafluoride
(SiF4) and hydrogen, in a capacitively-coupled plasma CVD system. The samples
used in this study were deposited on glass (Corning 7059), and conductivity
measurements were performed with aluminium electrodes in a coplanar geometry
*Paper presentedat the 7th International Conference on Thin Films, New Delhi, India, December 7 11,
1987.
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