550 IEEE ELECTRON DEVICE LETTERS, VOL. 30, NO. 5, MAY 2009
Stackable All-Oxide-Based Nonvolatile Memory
With Al
2
O
3
Antifuse and p-CuO
x
/n-InZnO
x
Diode
Seung-Eon Ahn, Bo Soo Kang, Ki Hwan Kim, Myoung-Jae Lee, Chang Bum Lee,
Genrikh Stefanovich, Chang Jung Kim, and Youngsoo Park
Abstract—We developed all-oxide-based nonvolatile memory
for low-cost, high-density, and high-performance one-time field-
programmable (OTP) memories compared with Si-based antifuse
memory using antifuse technologies over a glass substrate. The
oxide OTP memory employed the p-n CuO/InZnO
x
diode as the
switching element of the memory cell and Al
2
O
3
for the antifuse
as the storage node of the memory cell. The memory cell is pro-
grammed from the breakdown of Al
2
O
3
by applying a program
voltage bias that is about 4.5 V. The OTP memory cells show
large on/off ratio of about 10
6
and small current distributions at
programmed and unprogrammed states resulting from the perfect
uniformity of Al
2
O
3
thin film before and after breakdown. It also
showed a fast programming speed of about 20 ns.
Index Terms—Antifuse, one-time field-programmable (OTP)
memory, oxide diode.
I. I NTRODUCTION
R
ECENTLY, as the portable electronic equipment market
has remarkably grown, the demand for low-cost and
high-density nonvolatile memory has drastically increased. The
requirement for high-density memory has led to a consider-
able scaling of photolithography technology [1], [2]. Also, it
has brought novel nonvolatile memories and multilayer stack
structures for the advantage of high density per unit area
[3] as an alternative way to overcome technical and physical
limitations of 2-D scaling [4]–[6]. However, although high-
density nonvolatile memory using epitaxial or polycrystalline
silicon may be realized, it is difficult to meet the needs for
low cost due to high processing temperature and high man-
ufacturing cost. In addition, Si is not a proper material for
stacked structures. Because Si cannot be grown as a single
crystal over an arbitrary material and polycrystalline Si, devices
require high-temperature annealing that degrades or destroys
previously deposited layers and brings about unwanted layer
formation such as silicide on the metallic layer. In this point
of view, oxide materials may be better candidates for low-cost
and high-density nonvolatile memory because of their simple
growing process, availability of low-temperature growth, and
no restriction of substrate to Si [7]–[9].
In this letter, we have developed a stackable all-oxide-based
nonvolatile memory for low-cost and high-density one-time
Manuscript received January 22, 2009; revised February 19, 2009. First
published March 31, 2009; current version published April 28, 2009. The
review of this letter was arranged by Editor T. Wang.
The authors are with the Semiconductor Laboratory, Samsung Advanced
Institute of Technology, Yongin 449-711, Korea (e-mail: seungeon.ahn@
samsung.com; bosoo.kang@samsung.com).
Color versions of one or more of the figures in this letter are available online
at http://ieeexplore.ieee.org.
Digital Object Identifier 10.1109/LED.2009.2016582
Fig. 1. (a) Schematic diagram of an oxide p-n diode with antifuse cell. The
width of the bit line and word line is 0.5 μm. (b) Antifuse cross-point memory
was integrated on a glass substrate. (c) SEM image of 8 × 8 cross-point cell
array. The inset shows the SEM image of a 500 nm × 500 nm cross-point cell.
(d) High-resolution transmission electron microscopy cross-sectional image of
a 500 nm × 500 nm cell.
field-programmable (OTP) memories. Our oxide OTP memory
employed the p-n CuO/InZnO
x
diode as the switching element
of the memory cell to prevent reading interference between
neighboring cells and Al
2
O
3
for the antifuse as the storage node
of the memory cell. Antifuse technologies have been used for
OTP element in complex logic or memory ICs. The OTP mem-
ory employing an antifuse material generally programs two
logic states (“1” or “0”) of storage node using the breakdown of
antifuse. When the antifuse is in its pristine state, the memory
cell insulates the anode and the cathode, which means that no
significant current can flow. It is “1” state. When the antifuse is
ruptured by applying more than the breakdown voltage of the
antifuse, the memory cell is no longer insulating but shows a
diode characteristic only. It is “0” state. Our all-oxide-based
OTP memory using this typical antifuse program method is
free from thermal budget due to low process temperature and
shows excellent electrical characteristics compared with Si-
based OTP memories. The detailed device fabrication process
and the performance of the cells are described in this letter.
II. EXPERIMENTAL SETUP
Fig. 1(a) shows the schematic diagram of an oxide p-n diode
with an antifuse cell. Al
2
O
3
, a 2-nm-thick antifuse material,
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