SPECTROCHIMICA
ACTA
PART B
ELSEVIER Spectrochimica Acta Part B 52 (1997) 295-304
Analytical time-resolved laser enhanced ionization spectroscopy
I. Collisional ionization and photoionization of the Hg Rydberg states in
a low pressure gas
W.L. Clevenger, L.S. Mordoh, O.I. Matveev a, N. Omenetto 2, B.W. Smith,
J.D. Winefordner*
Department of Chemistry, University of Florida, Gainesville, FL 32611-7200, USA
Received 7 June 1996; accepted 4 September 1996
Abstract
The temporal behavior of the laser enhanced ionization signal of mercury was studied in a quartz cell under low buffer gas
pressure. Using fast electronics and a short (34 ns) laser pulse, it was possible to distinguish, in one single time-resolved
ionization waveform, the non-selective photoionization component of the signal from that which was due to collisional
ionization from selected levels. Experimental results were shown to agree with those obtained by computer simulation, and
optimal conditions for deconvolution of the two components were studied. © 1997 Elsevier Science B.V.
Keywords: Mercury; Time-resolved Ionization; Rydberg Levels; Photoionization; Collisional Ionization
I. Introduction
In laser enhanced ionization (LEI) spectroscopy
[1], the process of ion formation due to collisional
ionization of analyte atoms can practically always
be accompanied by their resonance photoionization
and by non-selective ionization of molecules and/or
atoms of buffer gas. Often, in order to improve the
limit of detection, one needs to acquire separate infor-
mation about the contribution of the LEI signal
bearing useful analytical information and the signal
due to non-selective photoionization. This subject has
been treated in several papers, together with the
* Corresponding author.
~On leave from Department of Chemistry, Moscow State
University, Moscow, Russia.
2 Present address: Environment Institute, Joint Research Centre,
Ispra, (Va) Italy.
different concepts associated with the two definitions
of ion yield and ionization efficiency [2-6]. Most
work has been performed in flames operated at
atmospheric pressure. Recently, it has been suggested
[7] that when using flames as atomizers, this informa-
tion can be obtained by observing a single time-
resolved ionization waveform under conditions
when the faster photoionization component and the
slower collisional ionization component of the signal
can be distinguished from one another. This idea can
be extended to other atom reservoirs, such as a low
pressure buffer gas. The deconvolution becomes pos-
sible when (1) the duration of the laser pulse is shorter
than the average time in the collisional ionization
process and (2) the distance between the collection
electrode and the laser beam is less than the average
distance traveled by the electron as a result of its drift
velocity during the process of the collisional
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