ANTIMICROBIAL AND ANTIOXIDANT ACTIVITY OF EMBLICA
EXTRACTS OBTAINED BY SUPERCRITICAL CARBON DIOXIDE
EXTRACTION AND METHANOL EXTRACTION
XIAOLI LIU
1,2
, MOUMING ZHAO
1,3
, JINSHUI WANG
1
and WEI LUO
1
1
College of Light Industry and Food Science
South China University of Technology
Guangzhou 510640, China
2
Faculty of Chemical Engineering and Light Industry
Guangdong University of Technology
Guangzhou 510006, China
Accepted for Publication August 6, 2007
ABSTRACT
This study is aimed to evaluate the antimicrobial and antioxidant activities
of two extracts of emblica (Phyllanthus emblica L.) obtained by supercritical
fluid extraction (SFE) and methanol extraction. The SFE extract showed strong
antimicrobial activity against all microorganisms tested, whereas the methan-
olic extract showed low activity against Staphylococcus aureus and fungi. In
contrast, the methanolic extract exhibited significantly higher antioxidant
activity than the SFE extract. The SFE extract was analyzed by gas chroma-
tography with mass spectrometric detector. Thirty compounds were tentatively
identified, representing 99.67% of the volatile components. b-Bourbonene,
teracosane, palmitic acid, thymol, b-caryophyllene and undecane were the
major compounds. The methanolic extract was subjected to separation and
purification using reverse-phase high-performance liquid chromatography.
Kaempferol 3-b-D-glucopyranoside (1), kaempferol (2), quercetin (3), isoco-
rilagin (4) and geraniin (5) respectively, were identified by spectral methods,
1
H
and
13
C nuclear magnetic resonance spectroscopy, ultraviolet-visible spectro-
photometry and mass spectroscopy, and comparison with literatures.
PRACTICAL APPLICATIONS
The study can be considered as the first report on the in vitro antimicro-
bial and antioxidant properties of supercritical fluid extraction (SFE) and
3
Corresponding author. TEL: +86-20-87113914; FAX: +86-20-87114954; EMAIL: femmzhao@
scut.edu.cn
Journal of Food Biochemistry 33 (2009) 307–330.
© 2009, The Author(s)
Journal compilation © 2009, Wiley Periodicals, Inc.
307