TIBS 18 - JULY 1993
example of mucins. Consequently, a func-
tional role in maintenance of surface
integrity, renewal and pathology of
mucous epithelia seems likely.
Acknowledgements
We thank Dr R. A. Hughes for critically
reading the manuscript. Our search for
new P-domains has been supported by
the 'Schilling-St[[tung'.
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Lateral communication by fast proton
conduction: a model membrane study
COMMUNICATION at the level of bio-
logical membranes is mainly described
as a trans phenomenon. In bioenergetic
terms, energy transduction is considered
to occur, mediated by transmembrane
proton gradientsL But on each inter-
[ace, the connection between pumps
and sinks is considered to be either
delocalized, i.e. occurring through the
bulk phase, or localized, i.e. along the
membrane' (Fig. I). The second case,
the so called 'microlocalized' chemi-
osmotic scheme, requires the existence
of 'protonic networks '2 that would link
pumps and sinks in small coupling units:L
Recently, direct experimental evidence
of the occurrence of such a lateral
transfer has been demonstrated with
model systems. Such a lateral transfer
of information along the membrane
may be a key process in biology.
Proton transfer: a physlcochemical
description
All theoretical descriptions of proton
conduction in biological systems are
derived from the Bjerrum-Eigen-
Onsager hypothesis 4 on the mechanism
of proton conduction in ice. The basic
J. Teissl6, B. Gabriel and M. Prats are at the
Department of Glycoconjugates and
Biomembranes, UPR8221 du CN S,
118 route de Narbonne,31062 Toulouse,
France.
© 1993, Elsevier 5c=ence Publishers, (UK) 0968-0004/93/$06.00
Lateral communication of information along biological membranes is thought
to be a key process for many cellular activities, Support for this hypothesis
comes from physicochemical experiments that show that an efficient fa-
cilitated lateral proton conduction exists along lipid-water interfaces. The
existence of a local two-dimensional hydrogen bond network between the
lipid headgroups and their associated water molecules would explain this
phenomenon.
idea is linked to the presence of hydro-
gen bonds between water molecules.
Two processes are involved: (1) a pro-
ton jumps from a 1130 ÷to a neighbouring
H~.O molecule (hopping step); (2) proro-
tational motion induces a small move-
ment of the involved protons in one
direction (Grotthus-type mechanism).
A similar transfer has been described
in biology. In the case of a proteinous
proton channel, the proton movement
was postulated to be due to the hydro-
gen bond network linking the amino
acids of the helix of a transmembra-
neous protein 5. Two steps are again
involved: (1) a hopping step where a
proton jumps from one side-chain
amino group, DH', to the neighbouring
one, A; (2) a reorientahon step of the
protonated acceptor AH ÷ through a flip-
flop process to give a new donor DW.
A more flexible network was pro-
posed where the proton transfer along
the proton channel was suggested to
involve a mixed linear hydrogen bond
system between amino acids and bound
water molecules6. Such a composite
network would allow (1) the adjust-
ment of the distance between the donor
and the acceptor of exchanged protons,
and (2) a faster rotation of the groups
than in a purely peptidic system. A
243