The processes of fusion-fission and quasi-fission of superheavy nuclei
M. G. Itkis
a
, A. A. Bogachev, I. M. Itkis, J. Kliman, G. N. Knyazheva,
N. A. Kondratiev, E. M. Kozulin, L. Krupa, Yu. Ts. Oganessian, I. V. Pokrovsky,
E. V. Prokhorova, A. Ya. Rusanov
a
Flerov Laboratory of Nuclear Reactions, JINR, 141980 Dubna, Russia
1. INTRODUCTION
One of the main problems of modern nuclear physics is the finding of extremal conditions
for the existence of atomic nuclei. The synthesis of new superheavy elements in heavy
ion induced reactions is an important part of these investigations. The survivability of
superheavy elements (SHE) with respect to the fission process is defined by the fission
barrier height, which completely depends on nuclear shells in the superheavy region. At
approaching the shell closure the fission barrier grows and the survivability of superheavy
nuclei increases. The recent success in the synthesis of new elements with Z = 112 - 118,
produced in the reactions with
48
Ca ions and actinide targets
238
U,
244
Pu,
248
Cm and
249
Cf [1,2], confirms the existence of “the island of stability” of SHE near the proton shell
closure with Z = 114, 120, 122 and neutron shell N = 184.
However, the fusion process of massive nuclei with heavy ions (A
i
≥ 27) differs greatly
from the reactions with more light ions, in which the fusion always occurs after the capture
stage. An increase in the Coulomb repulsion forces between interacting massive nuclei can
lead to the decay of the composite nuclear system before it reaches a compact shape near
the ground state. In this case the quasi-fission (QF) process [3,4] takes place. Quasi-fission
is a fast process and its experimental features differ from those of the true fusion-fission
(FF) process: large width of mass distributions, asymmetries in mass-angle correlation
of fragments and large angular anisotropies [5]. The neutron [6] and γ -multiplicities [7,8]
are also different in both processes. It has been found recently [9] that the total kinetic
energy (TKE) of fragments is higher in the QF process than that in the FF-process.
Different factors influence the FF/QF competition, such as the entrance channel mass
asymmetry, N/Z ratio, excitation energy and angular momentum, the deformation and
orientation of colliding nuclei, shell structure of the entrance channel and the formed
compound nucleus (CN).
It is well known that in heavy ion induced reactions leading to the formation of SHE
the deep-inelastic and quasi-fission processes are the dominant reaction channels, whereas
the fusion probability is much lower. In the reactions with
48
Ca-ions and actinide targets
the probability of fusion relative to QF is less than 10%, and the ratio decreases for more
symmetrical target-projectile combinations used in cold fusion reactions. The last SHE
which can be produced in the reaction with
48
Ca-ions is the element with Z = 118 since
the heaviest possible target is Cf. Thus to produce more heavy elements more heavy
Nuclear Physics A 787 (2007) 150c–159c
0375-9474/$ – see front matter © 2006 Elsevier B.V. All rights reserved.
doi:10.1016/j.nuclphysa.2006.12.026