Jointly published by React.Kinet.Catal.Lett.
Akadémiai Kiadó, Budapest Vol. 77, No. 2, 263-266
and Kluwer Academic Publishers, Dordrecht (2002)
0133-1736/2002/US$ 12.00.
© Akadémiai Kiadó, Budapest.
All rights reserved.
RKCL4065
Pt-Cu/ZSM-5 FOR REMOVAL OF NITRATES FROM DRINKING
WATER
Carolina Pfaff
a
, Luis Melo
a
and Paulino Betancourt
b
a
Departamento de Química Aplicada, Facultad de Ingeniería, Universidad Central de Venezuela,
Caracas, Venezuela
b
Centro de Catálisis, Petróleo y Petroquímica, Facultad de Ciencias, AP 47102. Los
Chaguaramos, Caracas, Venezuela. Tel.: 58-212-6051649. E-mail: pbetanco@strix.ciens.ucv.ve
Received January 28, 2002
In revised form June 4, 2002
Accepted June 17, 2002
Abstract
Removal of nitrates from drinking water by catalytic hydrogenation over ZSM-5
supported Pt-Cu catalysts was studied. Bimetallics Pt-Cu were prepared by ion
exchange of copper on a parent monometallic platinum catalyst. Monometallic
platinum catalysts are inactive for nitrate reduction, while Pt-Cu bimetallic
catalysts are active for nitrate removal. In the bimetallic catalyst, the role of
copper is probably to reduce nitrate according to a redox reaction. The addition of
copper to Pt catalysts decreases the production of ammonium ions
Keywords: Nitrates, reduction, Pt-Cu / ZSM-5 catalysts
INTRODUCTION
Nitrate is a commonly found contaminant in ground water, due to
agricultural, industrial and domestic practice. Excessive nitrate in drinking
water can cause methemoglobinemia in humans; the current drinking water
standard for nitrate (NO
3
-
- N) is 10 mg L
-1
. Therefore, there is a considerable
public interest and regulatory pressure to clean-up nitrate-contaminated
aquifers. In order to reduce the content of these pollutants in water, several
physico-chemical and biological processes have been proposed, such as ion
exchange, electrodialysis, reverse osmosis or microbiological treatment [1,2].