INTERNATIONAL JOURNAL OF PRECISION ENGINEERING AND MANUFACTURING Vol. 13, No. 12, pp. 2183-2186 DECEMBER 2012 / 2183
© KSPE and Springer 2012
Graphite Foil Based Assembled Bipolar Plates for
Polymer Electrolyte Fuel Cells
Sanghoon Ji
1
, Yong-Sheen Hwang
2
, Taehyun Park
3
, Yoon Ho Lee
3
, Jun Yeol Paek
3
,
Ikwhang Chang
1
, Min Hwan Lee
4
, and Suk Won Cha
3,#
1 Department of Intelligent Convergence Systems, Seoul National University, Daehak-dong, Gwanak-gu, Seoul, South Korea, 151-742
2 Fuel Cell Vehicle Team, Hyundai Motor Company, 104 Mabuk-dong, Giheung-gu, Yongin, South Korea, 446-912
3 School of Mechanical and Aerospace Engineering, Seoul National University, Daehak-dong, Gwanak-gu, Seoul, South Korea, 151-742
4 School of Engineering, University of California, Merced, 5200 North Lake Road, Merced, CA 95343, USA
# Corresponding Author / E-mail: swcha@snu.ac.kr, TEL: +82-2-880-8050, FAX: +82-2-880-1696
KEYWORDS: Assembled bipolar plate, Graphite foil, Polycarbonate, Current collector, Support, Polymer electrolyte fuel cell (PEFC)
Graphite foil has been considered as a promising bipolar plate material in polymer electrolyte fuel cells due to its high electrical
conductance and high corrosion resistance as well as low manufacturing costs. However, the highly flexible character of graphite foil
led to physical deformation under external mechanical and thermal stimuli during fuel cell operations. In this study, we show a
modified bipolar plate to overcome the weakness by combining with a mechanically sturdy component – polycarbonate plate. A unit
cell with the assembled bipolar plates showed stable powering behaviors under thermal cycling. There was no significant difference
in ohmic resistance between a unit cell with the assembled bipolar plates and a unit cell with graphite plates.
Manuscript received: July 2, 2012 / Accepted: August 17, 2012
1. Introduction
Polymer electrolyte fuel cells (PEFCs) have gained much attention
as a next-generation renewable energy conversion device due to their
high energy efficiency and low operating temperature.
1
By many
researches related to physical and chemical properties, an electro-
chemical performance of PEFCs reached close to the commercial level.
However, their high manufacturing cost is still impeding their active
commercialization.
2-6
Particularly, graphite plates widely used as separators
in PEFCs comprise more than 20% of the PEFC stack manufacturing
cost for large volume manufacturing.
7-9
Graphite foil has been considered a prospective bipolar plate material
due to the excellent electrical and thermal properties, and its low
manufacturing cost.
10,11
However, graphite foil bipolar plates can be easily
deformed by clamping forces applied to ensure decent fuel cell
performance.
12
Moreover, repetitive start and stop operations can cause
deformations of the bipolar plates, which result in non-uniform pressure at
the interface with the membrane electrode assembly (MEA).
13
Therefore,
it is highly required to find effective ways to prevent graphite foil from
being deformed by external mechanical and thermal stimuli.
In this study, we designed bipolar plates that are assembled by
combining graphite foils and polycarbonate plates. Graphite foil with
flow-fields acts as a current collector and polycarbonate plate supports
structure of the graphite foil. To investigate the effect of thermal cycle
on cell performance, start/stop operations were conducted for 3 days.
The feasibility of the assembled bipolar plate in PEFCs was studied by
comparing polarization and ohmic resistances of a unit cell with the
assembled bipolar plates (using a graphite foil) with those of a unit cell
with graphite bipolar plates only (we call it the reference cell).
2. Experimental Procedure
A unit cell having an active area of 25 cm
2
with membrane
electrode assembly (MEA; 7-layer series, 3 M Corp.) was clamped by
applying a torque of 30 kgf·cm and sealed with silicon-based sealants.
14
Heating of cells was carried out by conductive cartridge heater units.
Table 1 shows the experimental conditions and features of the MEA
used for the study. All MEAs were activated at 60
o
C for six hours with
fully humidified hydrogen and air, which allegedly caused little
changes in the voltage behaviors with test time until a performance
degradation occurred.
15
Custom-made station was used to evaluate
electrochemical performance of cells. Fig. 1 shows a schematic dia-
gram of the station. Fully humidified hydrogen and air were supplied
with a flow rate of 0.2 and 1.0 lpm, respectively.
The discharge of cells was controlled by direct current electronic loader
DOI: 10.1007/s12541-012-0289-7