Abstract— During irradiation tests at high temperature,
failure of commercial Inconel 600 sheathed thermocouples is
commonly encountered. To understand and remediate this
problem, out-of-pile tests were performed with thermocouples in
carburizing atmospheres which can be assumed to be at least
locally representative for High Temperature Reactors. The
objective was to screen those thermocouples which would
consecutively be used under irradiation. Two such screening tests
have been performed with a set of thermocouples embedded in
graphite (mainly conventional Type N thermocouples and
thermocouples with innovative sheaths) in a dedicated furnace
with helium flushing. Performance indicators such as thermal
drift, insulation and loop resistance were monitored and
compared to those from conventional Type N thermocouples.
Several parameters were investigated: niobium sleeves, bending,
thickness, sheath composition, temperature as well as the
chemical environment. After the tests, Scanning Electron
Microscopy (SEM) examinations were performed to analyze
possible local damage in wires and in the sheath. The present
paper describes the two experiments, summarizes results and
outlines further work, in particular to further analyze the
findings and to select suitable thermocouples for qualification
under irradiation
I. INTRODUCTION
HE main objective of High Temperature Reactor (HTR)
fuel irradiation tests in the High Flux Reactor Petten is to
check the feasibility of low coated fuel particle failure at high
temperatures and high burn-up [1][2][4]. To qualify this fuel
type, the irradiation campaigns (typically > 2 years at high
temperature exposure) must demonstrate effective fission
product retention under normal and off-normal operating
conditions.
Manuscript submitted May 20, 2011.
M. Laurie is with the European Commission, Joint Research Centre, Institute
for Energy, P.O. Box 2, NL-1755 ZG Petten (telephone: +31 224 565062, e-
mail: mathias.laurie@ec.europa.eu).
S. Fourrez is with THERMOCOAX SAS, BP 26, Planquivon, F-61438 Flers
Cedex, FR (telephone: +33 233 628119, e-mail:
stephane.fourrez@thermocoax.com).
M. A. Fütterer is with the European Commission, Joint Research Centre,
Institute for Energy, P.O. Box 2, NL-1755 ZG Petten (telephone: +31 224
565158, e-mail: michael.fuetterer@jrc.nl).
J. M. Lapetite is with the European Commission, Joint Research Centre,
Institute for Energy, P.O. Box 2, NL-1755 ZG Petten (telephone: +31 224
565159, e-mail: jean-marc.lapetite@ec.europa.eu).
In a pebble irradiation rig, in-pile instrumentation including
thermocouples, gamma scan wires and neutron fluence
detector sets has to find place in this narrow environment. In
such a rig, graphite structures are employed to hold the fuel in
place and to conduct the produced heat radially to the outside.
Real reactors use large amounts of graphite as moderator and
reflector material. The reaction of traces of water, trapped in
the graphite or imported by the purge gas, with the
carbonaceous material in the fuel element may lead to
appearance of reaction products such as CO, CO
2
, CH
4
and H
2
in the irradiation rig. Humidity is low in this environment, but
impurities (5 – 10 vppm) in the purge gas (a He/Ne mix) may
lead to reactions with the metallic sheath of the
thermocouples. This chemical contamination may react with
the built-in instrumentation and lead to severe corrosion or
carburization with thermocouples in contact with graphite.
Indeed, massive failures of Inconel 600 sheathed
thermocouples have been encountered during the HFR-EU1
irradiation test. Measurements showed significant drops in
insulation values on most thermocouples.
In order to prevent this situation in the future, two out-of-
pile tests were performed with a set of chosen thermocouples
mimicking as much as possible the environment encountered
by the in-core instrumentation. During these long-term
screening tests in representative conditions, the effects of
several parameters were investigated: niobium sleeves,
bending, thickness, sheath composition, temperature as well as
the chemical environment. The sets of thermocouples
embedded in graphite were tested in a dedicated furnace with
2.4 l/h helium flushing under 0.15 MPa at 1373 K and 1423 K.
The last part of the tests was performed with a purposely
contaminated helium atmosphere representative of the
atmosphere inside an irradiation rig with an initial content of
moisture assumed from degassing of graphite.
II. IN-PILE TESTS IN THE HFR
A. Background
The HFR is a multi-purpose research reactor which uses
light water as coolant and moderator. The normal operating
power is 45 MW. Special irradiation rigs have been developed
and are regularly used for testing fuel samples under
conditions which are representative of the current conditions
of the power plant[2][3]. A typical HTR fuel irradiation test is
Long Term out-of-pile Thermocouple Tests
in Conditions Representative for Nuclear
Gas-cooled High Temperature Reactors
M. Laurie, S. Fourrez, M. A. Fütterer, J. M. Lapetite,
T
978-1-4577-0927-2/11/$26.00 ©2011 IEEE