Pergamon
Tetrahedron 55 (1999) 1111-1118
TETRAHEDRON
Reaction of Diimines and Benzyne
Ashraf A. Aly, Nasr K. Mohamed, Alaa A. Hassan,
AbouI-Fetouh E. Mourad
Chemistry Department, Faculty of Science, EI-Minia University, EI-Minia, Egypt.
Received 1 July 1998; revised 6 November 1998; accepted 19 November 1998
Abstract: The reaction between benzyne and the Schiff bases la,b and 15a,b leads to the 1,4-bis(2 L
substituted acridin-10-yl)benzene 4a,b, the N-phenylarylamines 10a,b and the 10-(4 ~-formylphenyl)-substituted
acridines 1la,b (from ta,b) and the 2-substituted acridine-10-carboxyaldehyde18a,b (from 15a,b). Cyclohexyl
(4-cyclohexyliminomethylbenzyUdine)aminelc reacts with benzyne by an ene-reactionto give cyclohexenyl[(4-
cyclohexyliminomethylphenyl)benzylidine]amine 14. © 1999 ElsevierScience Ltd. All rightsreserved.
Introduction
The Diels-Alder reaction has been of prime importance in organic synthesis for a long
time 1-3, and among the numerous dienophiles employed arynes (dehydrobenzenes) have also been
added to a variety of dienes4's.
We are interested in preparing fused polycyclic compounds related to [2.2]paracyclophane using the
Diels-Alder reaction s'7, especially the reactions which involve benzyne as a dienophile8. Because of the
potential importance of the Diels-Alder reaction for the preparation of six-membered nitrogen
heterocycles, we try to utilize this reaction with benzyne to synthesize such nitrogen heterocycles which
have medicinal and industrial importance. Preparation of these compounds usually requires several steps
and proceeds with relatively poor yields.
The highly reactive parent system, benzyne, reacts with imines to give N-(o-anilinobenzhydryl)-
aniline 9 and phenanthridine derivatives 1 o as well as acridines 11 via [2+2] and/or [4+2] cycloaddition
reactions. Acridine derivatives have a wide range of applications in dye chemistry and are of medicinal
importance as antitumor reagents 12,13.
We have recently reported that cyclohexyl-(4-cyclohexyliminomethylbenzylidine)amine as well as
N,N~-bis-(aryl)-benzene-l,4-diylidmethylidenediamines react with tetracyanoethylene ('l'CNE),l,4-benzo-
and naphtho-quinone derivatives to give novel pyrrole, imidazolidine, quinoline, quinoxaline, indole
and carbazole derivatives 14As. On the other hand, 3,4,5,6-tetrachloro-l,2-benzoquinone (o-CHL)
provided a transient condensation product with the above diimines which underwent [4+2] cycloaddition
0040-4020/99/$ - see front matter © 1999 Elsevier Science Ltd. All rights reserved.
PII: S0040-4020(98)01089-8